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Record W4292510267 · doi:10.1002/cem.3439

A Raman spectroscopy–compositional–structural investigation of lunar surface materials and analogues

2022· article· en· W4292510267 on OpenAlexafffund
E. A. Cloutis, Nathalie Turenne, Sahejpal Sidhu, Stephanie Connell, D. M. Applin

Bibliographic record

VenueJournal of Chemometrics · 2022
Typearticle
Languageen
FieldPhysics and Astronomy
TopicPlanetary Science and Exploration
Canadian institutionsUniversity of Winnipeg
FundersNatural Sciences and Engineering Research Council of CanadaCanadian Space AgencyCanada Foundation for InnovationUniversity of Winnipeg
KeywordsRaman spectroscopyEnstatitePlagioclaseForsteriteOlivineMeteoriteContext (archaeology)MineralAnalytical Chemistry (journal)GeologyPyroxeneMineralogyMelt inclusionsMaterials scienceChemistryQuartzAstrobiologyPhysicsChondriteOptics

Abstract

fetched live from OpenAlex

Abstract We investigated the Raman spectroscopy of 35 rock and mineral samples of composition relevant to the lunar surface: pyroxenes, olivine, plagioclase feldspars and oxides. The Raman spectra were analysed in the context of their compositional and structural properties to develop robust correlations to enable their detection on the lunar surface by Raman spectroscopy. We developed and implemented a spectral deconvolution program to model the fluorescence background and various Raman peaks to extract their positions in wavenumber space. Relations were developed between the Raman peak positions of pyroxenes around 325, 670 and 1000 cm −1 with their compositions in terms of enstatite, ferrosilite and wollastonite components. For olivines, we verified previously determined correlations between the positions of the olivine‐related peak doublet between 800 and 880 cm −1 with forsterite content. We also discuss the main signatures detected in the Raman spectra of plagioclases and oxides. The derived relationships were examined using Raman spectra of the matrix and several inclusions of the lunar meteorite NWA12593. We were able to identify the main endmembers of the selected surface spots as pyroxenes, plagioclase feldspars and olivine. We used the previous correlations to separate orthopyroxene from clinopyroxene signatures and to propose a composition of the inclusions of the meteorite. The results of this study demonstrate the utility of Raman spectroscopy for determining the mineralogy of the lunar surface.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.230
Teacher spread0.216 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations8
Published2022
Admission routes2
Has abstractyes

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