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Record W4295339159 · doi:10.1002/celc.202200717

Iron and Nickel Phthalocyanine‐Modified Nanocarbon Materials as Cathode Catalysts for Anion‐Exchange Membrane Fuel Cells and Zinc‐Air Batteries**

2022· article· en· W4295339159 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueChemElectroChem · 2022
Typearticle
Languageen
FieldEnergy
TopicElectrocatalysts for Energy Conversion
Canadian institutionsSimon Fraser University
FundersEuropean Regional Development FundEesti TeadusagentuurAgence Nationale de la Recherche
KeywordsCatalysisBimetalBimetallic stripCarbon fibersMaterials scienceCarbon nanotubeInorganic chemistryNickelPhthalocyanineGrapheneChemical engineeringAnodeCathodeRotating ring-disk electrodeChemistryElectrocatalystElectrodeNanotechnologyComposite numberElectrochemistryOrganic chemistryComposite materialMetallurgyPhysical chemistry

Abstract

fetched live from OpenAlex

Abstract Iron and nickel phthalocyanines along with different carbon supports, i. e., multi‐walled carbon nanotubes (MWCNT), graphene, carbide‐derived carbon, Vulcan carbon, and mesoporous carbon (MC, from Pajarito Powder, LLC), are used to prepare six bimetallic (Fe, Ni) N‐doped carbon‐based catalysts. The aim of this work is to investigate the electrocatalytic activity of bimetal phthalocyanine‐modified nanocarbon catalysts, e. g., the effect of carbon supports on the oxygen reduction reaction (ORR) and oxygen evolution reaction (OER), including the anion‐exchange membrane fuel cell (AEMFC) and rechargeable zinc‐air battery (RZAB) configuration. The catalysts exhibit excellent electrocatalytic activity as exemplified by their half‐wave potential ( E 1/2 ) for ORR and the potential at which the OER current density reaches 10 mA cm −2 ( E j =10 ), but the best performing catalysts are FeNiN−MC ( E 1/2 =0.88 V, E j =10 =1.58 V) and FeNiN−MWCNT ( E 1/2 =0.87 V, E j =10 =1.59 V). In AEMFC analyses, FeNiN−MWCNT cathode provides peak power density ( P max ) of 406 mW cm −2 , slightly higher than that of FeNiN−MC ( P max =386 mW cm −2 ). Both catalysts exhibit a good RZAB performance ( P max of 85 mW cm −2 for FeNiN−MWCNT). The assembled RZABs run stably for 48 h without any significant loss of performance.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.016
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.217
Teacher spread0.208 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it