MétaCan
Menu
Back to cohort

Overview of methods to characterize the mass, size, and morphology of soot

2023· article· en· W4379184168 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueJournal of Aerosol Science · 2023
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicAtmospheric chemistry and aerosols
Canadian institutionsUniversity of British ColumbiaUniversity of AlbertaNational Research Council Canada
FundersNational Research Council CanadaRoyal SocietyNational Aeronautics and Space AdministrationU.S. Department of EnergyNational Science Foundation
KeywordsSootAerosolFractal dimensionFractalCharacterization (materials science)Particle (ecology)Particle sizeMaterials scienceAggregate (composite)NanoparticleNanotechnologyLight scatteringBiological systemCombustionScatteringChemical physicsStatistical physicsChemistryOpticsPhysicsGeologyMeteorologyMathematics

Abstract

fetched live from OpenAlex

Combustion and other high-temperature processes can produce solid aerosol nanoparticles with complex morphologies, including fractal-like aggregates of primary particles. Characterizing these morphologies, as well as particle mass, is key to understanding their behavior in natural and engineered systems, and it can provide clues to the origin of the particles. We focus here on the characterization of soot, although most of the techniques apply to other aerosol aggregates. A complete description of these aerosols would include the mass and morphology of every particle. In practice, it is possible to obtain detailed information on individual particles from microscopy of extracted samples. A particular focus of this review, tandem classifier/detector systems can determine 2-dimensional mass and mobility distributions that may be interpreted through the lens of fractal models. Very fast in situ light scattering measurements can be used to determine the structure factor, related to fractal dimension, and the aggregate and primary particle size distributions. These approaches are complementary when there are appropriate models to connect morphological details to optical and transport characteristics of the particles. Over the last few decades these models have become more sophisticated, requiring more information on the particle structure and properties, but also facilitating more sophisticated inferences from in-situ and online measurement techniques.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.455
Threshold uncertainty score0.397

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.059
GPT teacher head0.328
Teacher spread0.269 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it