MétaCan
Menu
Back to cohort
Record W4386034573 · doi:10.1016/j.xcrp.2023.101548

Base metal chemistry and catalysis

2023· article· en· W4386034573 on OpenAlexafffund
Marissa L. Clapson, Connor S. Durfy, Devon Facchinato, Marcus W. Drover

Bibliographic record

VenueCell Reports Physical Science · 2023
Typearticle
Languageen
FieldEnergy
TopicCO2 Reduction Techniques and Catalysts
Canadian institutionsUniversity of Windsor
FundersNatural Sciences and Engineering Research Council of CanadaAmerican Chemical Society Petroleum Research FundCanada Foundation for InnovationCouncil of Ontario UniversitiesUniversity of Windsor
KeywordsCatalysisBase metalChemistryMetalBase (topology)Organic chemistryMaterials scienceMetallurgyMathematics

Abstract

fetched live from OpenAlex

This perspective provides an entry-level conversation concerning base metal catalysis as a green and sustainable solution in industrial and academic contexts. We establish a definition of “base metal,” challenging readers to consider the ethical implications of metal sourcing. We explore what it means to be “sustainable” and provide information on current efforts in synthetic chemistry. We provide examples of current catalytic trends and transformations in popular fields such as cross-coupling and small-molecule conversion, highlighting relevant base metal systems. Finally, we consider social context—for example, decisions related to catalyst development are often driven by factors including costliness, safety, social adoptability (whether society will accept its usage), and performance. How do we move base metal catalysis to the forefront? Is society concerned if materials are fabricated from cheaper and more abundant sources? How does the synthetic chemistry community guide this knowledge translation?

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.002
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.008
Threshold uncertainty score0.031

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0020.002
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0010.001
Science and technology studies0.0020.010
Scholarly communication0.0060.006
Open science0.0020.003
Research integrity0.0060.006
Insufficient payload (model declined to judge)0.0080.003

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.247
Teacher spread0.238 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations34
Published2023
Admission routes2
Has abstractyes

Explore more

Same venueCell Reports Physical ScienceSame topicCO2 Reduction Techniques and CatalystsFrench-language works237,207