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Record W4386046982 · doi:10.1039/d3cs00453h

A beginners guide to understanding the mechanisms of photochemical reactions: things you should know if light is one of your reagents

2023· review· en· W4386046982 on OpenAlexafffund
J. C. Scaiano

Bibliographic record

VenueChemical Society Reviews · 2023
Typereview
Languageen
FieldChemistry
TopicRadical Photochemical Reactions
Canadian institutionsUniversity of Ottawa
FundersNatural Sciences and Engineering Research Council of CanadaCanada Research Chairs
KeywordsReagentPopularityPhotochemistryChemistryComputer scienceCombinatorial chemistryOrganic chemistryPolitical scienceLaw

Abstract

fetched live from OpenAlex

The increasing popularity of applied photochemistry has changed the composition of the practitioners of photochemistry, from traditional specialists, to users whose expertise lies elsewhere, yet they find light as a useful and powerful reagent. I introduce Kasha's rule very early in this tutorial; this unconventional approach allows me to bypass information about high electronic states in favor of the lowest singlet and triplet excited states. Doing this I try to provide a fast entry enabling newcomers in the field of applied photochemistry to have a taste of what the field has to offer, in the hope that they will like what they see, and venture further into the many resources available to go deeper into the fascinating field of organic photochemistry.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.002
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: Not applicable
GenreCandidate signal: Review · Consensus signal: Review
Teacher disagreement score0.068
Threshold uncertainty score0.227

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.002
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0020.002
Science and technology studies0.0010.001
Scholarly communication0.0020.004
Open science0.0020.001
Research integrity0.0020.004
Insufficient payload (model declined to judge)0.0680.075

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.205
GPT teacher head0.394
Teacher spread0.189 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designNot applicable
Domainnot available
GenreReview

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations72
Published2023
Admission routes2
Has abstractyes

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