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Record W4391610858 · doi:10.1002/xrs.3418

Determination of trace elements in titanium oxides by wavelength dispersive x‐ray fluorescence spectrometry (WD‐XRF)

2024· article· en· W4391610858 on OpenAlexaboutno aff
M. F. Gazulla, M. Orduña, Marta Rodrigo

Bibliographic record

VenueX-Ray Spectrometry · 2024
Typearticle
Languageen
FieldChemistry
TopicAnalytical chemistry methods development
Canadian institutionsnot available
FundersInstituto Valenciano de Competitividad Empresarial
KeywordsCosmeticsX-ray fluorescenceMaterials sciencePelletsDetection limitIngredientTrace elementTRACE (psycholinguistics)ContaminationTitaniumEnvironmental chemistryMetallurgyChemistryFluorescenceChromatographyComposite material

Abstract

fetched live from OpenAlex

Abstract TiO 2 is used in a great variety of industries (foods, medicines, cosmetics, etc.). In food industry, although the use of TiO 2 as additive was banned by EU in 2022, it is still authorized in medicinal products, and is allowed as food ingredient in US and Canada. Focusing on cosmetics, regulations state some forbidden elements (As, Cd, Ni, Hg, Sb, and Pb), and others allowed with a specific limit (Co, Cr, and Se). Most researches about TiO 2 characterization are focused on the purity determination and no studies analyzing trace metals in this material have been found. Due to the potential impact of those trace elements on health and safety, a robust method for determining them in TiO 2 is required. A methodology for the determination of As, Cd, Co, Cr, Hg, Ni, Pb, Sb, and Se at trace level in TiO 2 by WD‐XRF has been developed. Sample was prepared as pressed pellets to achieve low limits required by regulations, and the best conditions were established using n‐butyl methacrylate as binder and plastic spatula to avoid Cr contamination coming from the stainless‐steel one. An in‐depth inquiry conducted to get calibration and validation standards revealed a lack of reference materials; therefore, additions of pure oxides of each element were made to high‐purity TiO 2 . Validation was performed by two means: analyzing synthetic standards prepared as stated and analyzing two commercial TiO 2 by an independent method (ICP‐OES). The developed methodology was suitable to be used as control method to assess whether the materials meet the regulations, since time required to undertake the analysis is much less than other methods.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.004

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.277
Teacher spread0.265 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2024
Admission routes1
Has abstractyes

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