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Record W4394789657 · doi:10.1016/j.surfin.2024.104282

TiO2-NPs/ZnO-NPs@Co3O4 nanocomposite from natural extracts for the Rhodamine 6 G photodegradation

2024· article· en· W4394789657 on OpenAlexaff
Robson Dias Wouters, Daniel Moro Druzian, Pâmela Cristine Ladwig Muraro, Maurício Dalla Costa Rodrigues da Silva, Claudinei dos Santos, Yolice Patricia Moreno Ruiz, André Galembeck, Giovani Pavoski, Denise Crocce Romano Espinosa, William Leonardo da Silva

Bibliographic record

VenueSurfaces and Interfaces · 2024
Typearticle
Languageen
FieldEnergy
TopicTiO2 Photocatalysis and Solar Cells
Canadian institutionsUniversity of British Columbia
FundersFundação de Amparo à Pesquisa do Estado do Rio Grande do Sul
KeywordsMaterials sciencePhotodegradationNanocompositeRhodamine BRhodamineNanoparticleChemical engineeringNuclear chemistryPhotocatalysisNanotechnologyOrganic chemistryFluorescenceOpticsCatalysis

Abstract

fetched live from OpenAlex

Socio-environmental issues are frequent in industrial growth, especially wastewater containing dyes resulting in toxic effects on fauna and flora. Parallelly, synthesizing nanomaterials using extracts allows for improved properties with fewer environmental effects. In this way, the present study aims to synthesize using natural extracts and characterize a ceramic nanocomposite containing titanium and zinc dioxide doped with tricobalt tetroxide nanoparticles (TiO 2 NPs/ZnO NPs@Co 3 O 4 NPs) for the removal of Rhodamine 6 G under visible radiation. TiO 2 -NPs/ZnO-NPs@Co 3 O 4 -NPs ceramic nanocomposite showed a heterogeneous morphology with a negative charge surface of -16.73 mV, V-type isotherm and H1 hysteresis, surface area (S BET ) of 62.2 m² g −1 , pore diameter (Dp) of 10.41 nm and bang gap energy (Eg) of 2.98 eV. The ideal condition of photocatalytic heterogeneous was of [Rh 6 G] = 3.18 mg L −1 , [NPs] = 1 g L −1 and pH = 7 with 99.97 % for the Rh 6 G photodegradation and the apparent rate of the pseudo first-order reaction ( k ) of 0.0193 min −1 . After IV cycles of TiO 2 -NPs/ZnO-NPs@Co 3 O 4 -NPs, there was a small reduction in Rh 6 G dye removal (99.97 to 85.71 %), confirming the photocatalytic stability of the nanocatalyst. Ecotoxicity tests were carried out with Lactuca sativa seeds and demonstrated root radicular inhibition of 6.41 % to 20.73% ranging from 12.5 - 100 mg L −1 . Machine Learning (ML) study was used to predict the Rh 6 G photodegradation mechanism, where the dye molecules successively cleavage such aromatic structure and carbonic acid to produce smaller fragments that are further form CO 2 and H 2 O. Therefore, ceramic nanocomposite presents potential application as a nanocatalyst for the wastewater treatment.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.254
Teacher spread0.240 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations28
Published2024
Admission routes1
Has abstractyes

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