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Record W4396720092 · doi:10.1021/acsestwater.3c00780

High-Frequency Data Provides Insight into Chloride Transport Pathways and Exceedances of Chronic Chloride Guidelines for the Protection of Aquatic Life in Streams Impacted by Deicers

2024· article· en· W4396720092 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.
aboutThe title or abstract carries a Canadian signal from the geographic lexicon.

Bibliographic record

VenueACS ES&T Water · 2024
Typearticle
Languageen
FieldEnvironmental Science
TopicSmart Materials for Construction
Canadian institutionsEnvironment and Climate Change CanadaToronto Metropolitan University
FundersNatural Sciences and Engineering Research Council of CanadaEnvironment and Climate Change Canada
KeywordsSTREAMSChlorideEnvironmental scienceEnvironmental chemistryChemistryComputer scienceOrganic chemistry

Abstract

fetched live from OpenAlex

Assessments of elevated stream chloride (Cl) concentrations ([Cl]), predominantly sourced from winter application of road deicers across snow belt regions, are starting to use high-frequency data, more so in the United States (U.S.) than in Canada. Here, [Cl] was derived from high-frequency specific conductance (SC) measurements from nine streams draining urbanized subwatersheds around Hamilton, Ontario, Canada, between May 2020 and April 2021. We assess [Cl] dynamics to understand dominant transport pathways and characterize water quality guideline exceedances to assess ecological risk while comparing Canadian and U.S. methodologies. These streams exhibited an alarming extent of high [Cl] as six streams exceeded the Canadian short-term guideline >90% of both the salting and non-salting seasons. High-frequency stream [Cl] revealed Cl-impacted groundwater maintaining baseflow [Cl], while fast pathways (e.g., sewers) drive [Cl] pulses in the salting season and episodic dilutions in the non-salting season. Application of the higher U.S. guideline gave consistently lower exceedances. Its application of rolling averages to high-frequency data also obscures episodic dilutions that reduce [Cl] below guideline thresholds and may provide brief intervals of refuge to organisms. High-frequency data provided insight into Cl pathways and ecological risk, though exceedance results are sensitive to the guideline methodology.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.014
Threshold uncertainty score0.988

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.037
GPT teacher head0.259
Teacher spread0.223 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it