MétaCan
Menu
Back to cohort
Record W4405131925 · doi:10.29173/eureka28818

Representing The World Around Us: Applications of Group Representation Theory to Molecular Orbital (MO) Theory

2024· article· en· W4405131925 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
venuePublished in a venue whose home country is Canada.

Bibliographic record

VenueEureka · 2024
Typearticle
Languageen
FieldChemistry
TopicHistory and advancements in chemistry
Canadian institutionsUniversity of Calgary
Fundersnot available
KeywordsGroup (periodic table)Molecular orbital theoryRepresentation theoryRepresentation (politics)Group representationMolecular orbitalTheoretical physicsPhysicsMathematicsPure mathematicsQuantum mechanicsMoleculePolitical science

Abstract

fetched live from OpenAlex

Molecular orbital (MO) theory is a theory at the forefront of modern chemistry, allowing for accurate descriptions of reactivity of molecules by using quantum mechanics to predict the location of electrons within a molecule, and their corresponding energies. The equations which govern their behavior, the Schrodinger equation, are often difficult to solve. Often, we can only approximate a solution using numerical methods. This paper discusses a method which exploits a molecule’s internal symmetry. Specifically, we use Group representation theory to help analyze and break down the molecular symmetry, and then use the analysis to help us find the MO’s. First, we establish key results about irreducible representations and characters. We then establish a correspondence between MO’s and irreducible representations. We then use the results we obtained to perform MO calculations on water (H2O). We then compare the results obtained via our MO theory calculations and Valance Bond Theory (VBT). We conclude by showing these calculations are best used for rough work, being most useful for deciding which atomic orbitals they arose from, and each MO’s energies relative to each other.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.597
Threshold uncertainty score0.919

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.294
Teacher spread0.283 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it