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Record W4406610724 · doi:10.1016/j.fuel.2025.134445

Life cycle GHG emissions assessment of vanadium recovery from spent catalysts from bitumen upgraders

2025· article· en· W4406610724 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueFuel · 2025
Typearticle
Languageen
FieldEngineering
TopicExtraction and Separation Processes
Canadian institutionsUniversity of Alberta
FundersNatural Sciences and Engineering Research Council of CanadaEnvironment and Climate Change CanadaCanada First Research Excellence FundCanada Research ChairsNatural Resources CanadaUniversity of AlbertaAlberta InnovatesCenovus EnergyCanada Excellence Research Chairs, Government of CanadaSuncor Energy Incorporated
KeywordsVanadiumAsphaltLife-cycle assessmentEnvironmental scienceGreenhouse gasEnvironmental chemistryCatalysisWaste managementGlobal-warming potentialChemistryMaterials scienceMetallurgyProduction (economics)EngineeringGeologyOrganic chemistryEconomics

Abstract

fetched live from OpenAlex

Bitumen from oil sands is a key source of fossil fuels. Bitumen is upgraded to produce synthetic crude oil, which is subsequently refined. The amount of vanadium in bitumen upgrading spent catalyst is substantial. Vanadium plays a vital role in steel production, chemical processes, and energy storage through its use in batteries, making it a valuable commodity worldwide. Recovering this metal from bitumen can be a profitable activity that could help contribute to global demand. Besides the economics of the process, the environmental impact should be addressed. However, details on the greenhouse gas (GHG) emissions generated during the process are not available. Therefore, we conducted a life cycle assessment of recovering vanadium from spent catalyst generated during bitumen upgrading. We developed a data-intensive model to estimate the GHG emissions from each life cycle stage of vanadium recovery from bitumen upgraders. The estimated life cycle GHG emissions are 11.8 kg CO 2 eq/kg V 2 O 5 . Of the total GHG emissions, 69 % are indirect and 31 % are direct emissions. If we consider the displacement of co-produced metals like molybdenum and alumina, the life cycle GHG emissions of the production system would drop to 0.63 kg CO 2 eq/kg V 2 O 5 . Sensitivity and uncertainty analyses show that the emission factor of electricity production, the specific energy consumption in the electric arc furnace, and the salt-to-spent catalyst ratio are the parameters with the most significant impact on the GHG emissions. Coupling a vanadium recovery plant with a bitumen upgrader is worthy of consideration because of the potential environmental benefits of the process.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: Not applicable
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.453
Threshold uncertainty score0.672

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.273
Teacher spread0.261 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it