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Record W4406610724 · doi:10.1016/j.fuel.2025.134445

Life cycle GHG emissions assessment of vanadium recovery from spent catalysts from bitumen upgraders

2025· article· en· W4406610724 on OpenAlexafffund
Miguel Baritto, A.O. Oni, Amit Kumar

Bibliographic record

VenueFuel · 2025
Typearticle
Languageen
FieldEngineering
TopicExtraction and Separation Processes
Canadian institutionsUniversity of Alberta
FundersNatural Sciences and Engineering Research Council of CanadaEnvironment and Climate Change CanadaCanada First Research Excellence FundCanada Research ChairsNatural Resources CanadaUniversity of AlbertaAlberta InnovatesCenovus EnergyCanada Excellence Research Chairs, Government of CanadaSuncor Energy Incorporated
KeywordsVanadiumAsphaltLife-cycle assessmentEnvironmental scienceGreenhouse gasEnvironmental chemistryCatalysisWaste managementGlobal-warming potentialChemistryMaterials scienceMetallurgyProduction (economics)EngineeringGeologyOrganic chemistryEconomics

Abstract

fetched live from OpenAlex

Bitumen from oil sands is a key source of fossil fuels. Bitumen is upgraded to produce synthetic crude oil, which is subsequently refined. The amount of vanadium in bitumen upgrading spent catalyst is substantial. Vanadium plays a vital role in steel production, chemical processes, and energy storage through its use in batteries, making it a valuable commodity worldwide. Recovering this metal from bitumen can be a profitable activity that could help contribute to global demand. Besides the economics of the process, the environmental impact should be addressed. However, details on the greenhouse gas (GHG) emissions generated during the process are not available. Therefore, we conducted a life cycle assessment of recovering vanadium from spent catalyst generated during bitumen upgrading. We developed a data-intensive model to estimate the GHG emissions from each life cycle stage of vanadium recovery from bitumen upgraders. The estimated life cycle GHG emissions are 11.8 kg CO 2 eq/kg V 2 O 5 . Of the total GHG emissions, 69 % are indirect and 31 % are direct emissions. If we consider the displacement of co-produced metals like molybdenum and alumina, the life cycle GHG emissions of the production system would drop to 0.63 kg CO 2 eq/kg V 2 O 5 . Sensitivity and uncertainty analyses show that the emission factor of electricity production, the specific energy consumption in the electric arc furnace, and the salt-to-spent catalyst ratio are the parameters with the most significant impact on the GHG emissions. Coupling a vanadium recovery plant with a bitumen upgrader is worthy of consideration because of the potential environmental benefits of the process.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.047
Threshold uncertainty score0.094

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.002
Bibliometrics0.0010.001
Science and technology studies0.0000.000
Scholarly communication0.0010.001
Open science0.0010.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.273
Teacher spread0.261 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2025
Admission routes2
Has abstractyes

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