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Record W4412932992 · doi:10.1021/acssusresmgt.5c00136

Liquids and Microbial Electrolysis Cells for Boosted CO<sub>2</sub> Methanogenesis: Role of Interfacial Electron Transfer

2025· article· en· W4412932992 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueACS Sustainable Resource Management · 2025
Typearticle
Languageen
FieldEnvironmental Science
TopicMicrobial Fuel Cells and Bioremediation
Canadian institutionsBiotechnology Research InstituteNational Institute for NanotechnologyUniversity of Waterloo
FundersNational Key Research and Development Program of ChinaNational Natural Science Foundation of China
KeywordsMethanogenesisElectrolysisElectron transferChemical engineeringChemistryElectronMaterials scienceEnvironmental chemistryChemical physicsMethanePhotochemistryElectrodeOrganic chemistryPhysicsPhysical chemistryEngineering

Abstract

fetched live from OpenAlex

High Resolution Image Download MS PowerPoint Slide This study explores the improvement of CO 2 methanogenesis using microbial electrolysis systems (MESS) and ionic liquids (ILs). The microbial community adapted to CO 2 methanogenesis showed performance enhancement over time, achieving 0.46 mmol/cycle of specific methane production in the combined MESS and IL system, while it was around 0.28 mmol/cycle for MES only. Under non-electrified conditions, methane production was quite lower (0.1 mmol/cycle). The highest CO 2 conversion efficiency was achieved in the MESS/IL (M-I-E) group, followed by microbiology (M), MESS/IL (M-I), and MESS(M-E). ILs enhanced the electrochemical activity of MESS, resulting in a higher current to 0.61 ± 0.05 mA and a higher Coulombic efficiency to 68.8 ± 3%, compared to 0.45 ± 0.05 mA and 55.6 ± 2% for MESS alone. Further evidence for the improvements was shown by the reduced charge transfer resistance (2.37 ± 0.08 Ω) and enhanced biomass accumulation at the cathode. The microbial community analysis pointed out a significant shift in dominant species, including a significant increase in methanogens such as Methanobacterium sp. and Methanoculleus bourgensis . Metabolic responses showed upregulation of key genes involved in the transporters, Wood–Ljungdahl pathway, and tricarboxylic acid (TCA) cycle, indicating that IL layers could provide channels directly or through outside cellular entities for electrons to efficiently shuttle for enhanced methanogenesis. These findings gain insights into the synergistic benefits of ILs and MESS in boosting CO 2 methanogenesis and provide insights into the underlying mechanisms.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.128
Threshold uncertainty score0.876

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.002
GPT teacher head0.191
Teacher spread0.188 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it