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Exploring sustainable lithium iron phosphate cathodes for Li-ion batteries: From mine to precursor and cathode production

2025· article· en· W4413014274 on OpenAlexafffund
Mehrdad Dorri, Atiyeh Nekahi, Sabbir Ahmed, Jeremy I. G. Dawkins, Thiago Matheus Guimarães Selva, Anil Kumar M R, Karim Zaghib

Bibliographic record

VenueJournal of Power Sources · 2025
Typearticle
Languageen
FieldEngineering
TopicExtraction and Separation Processes
Canadian institutionsConcordia University
FundersConcordia University
KeywordsCathodeLithium iron phosphateLithium (medication)Iron phosphatePhosphateIonProduction (economics)Inorganic chemistryLithium vanadium phosphate batteryChemistryMaterials scienceElectrodeAnodeElectrochemistryOrganic chemistry

Abstract

fetched live from OpenAlex

Lithium iron phosphate (LFP) cathodes are gaining popularity because of their safety features, long lifespan, and the availability of raw materials. Understanding the supply chain from mine to battery-grade precursors is critical for ensuring sustainable and scalable production. This review provides a comprehensive overview of the mining, beneficiation, processing, and purification processes of phosphorus, iron, and lithium ores. It explains the journey from mineral ores to purified iron (≥99 wt%) and phosphoric acid (≥85 wt%), detailing the strategies required to meet battery-grade specifications. This review covers different purification technologies and the key parameters that influence material grade and impurity levels. Processes capable of achieving impurity removal efficiencies of up to 99.9–100 % are highlighted. Although battery recycling has a high potential for recovering the material, existing extraction and refining processes for ores still need to be optimized to make processes both more efficient and more environmentally friendly. This review also discusses several production pathways for iron phosphate (FePO 4 ) and iron sulfate (FeSO 4 ) as key iron precursors. These insights are important for guiding future efforts toward the sustainable, efficient, and large-scale production of LFP cathodes to support the global energy transition. • Transformation of lithium, iron, and phosphorus ores into battery-grade precursors. • Key steps in purification and refining processes. • Overview of sustainable purified phosphoric acid production. • Methods to produce battery-grade Fe powder, Fe 2 O 3 /Fe 3 O 4 , FePO 4 , and FeSO 4 .

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.001
Threshold uncertainty score0.005

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.001
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0010.002
Open science0.0010.001
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0010.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.026
GPT teacher head0.263
Teacher spread0.236 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations11
Published2025
Admission routes2
Has abstractyes

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