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Controlling collagen I orientation on polyetheretherketone implants to improve epithelial sealing

2025· article· en· W4414085528 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueACS Biomaterials Science & Engineering · 2025
Typearticle
Languageen
FieldDentistry
TopicDental materials and restorations
Canadian institutionsMcGill University
FundersFonds de Recherche du Québec - SantéFonds Québécois de la Recherche sur la Nature et les TechnologiesNatural Sciences and Engineering Research Council of CanadaCanada Research Chairs
KeywordsIntegrinAdhesionSurface modificationCell adhesionCovalent bondExtracellular matrixCellHaCaT

Abstract

fetched live from OpenAlex

Transcutaneous devices such as dental implants frequently fail due to infections at their interfaces with epithelial tissues. These infections are facilitated by the lack of integration between the devices and the surrounding soft tissues. This study aims to improve epithelial integration through surface modification of a transcutaneous implant material (polyetheretherketone (PEEK)). The modification involved covalent bonding of collagen via two distinct methods: (1) nonselective binding through any primary amines present on collagen using carbodiimide-based coupling and (2) site-specific binding to the free amine on the N-terminus of collagen molecules. The second approach preserves active sites responsible for interacting with integrins, crucial for epithelial cell adhesion, located near the C terminus. Both conjugation methods resulted in similar amounts of immobilized collagen; yet, surfaces with 2-PCA-based collagen conjugation exhibited 4 times more free amines. This indicates that fewer amines were used for conjugation in these samples, confirming that 2-PCA selectively binds collagen only through the N-terminus amines. Collagen-conjugated surfaces significantly enhanced HaCaT epithelial cell viability and adhesion compared to unmodified PEEK. Furthermore, 2-PCA-based conjugation resulted in a 2-fold increase in β4 subunit gene expression of integrin α6β4 (a key epithelial cell adhesion marker), higher integrin β4 immunofluorescence (IF) intensity, and over a 30% improvement in cell retention following mechanical detachment, compared to nonselective conjugation. These findings suggest that selective collagen conjugation on PEEK surfaces increases the accessibility of collagen domains responsible for binding with integrin receptors, which in turn improves epithelial cell attachment, offering a promising strategy for reducing infections and enhancing the longevity of transcutaneous devices.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.012
Threshold uncertainty score0.735

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0010.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.281
Teacher spread0.273 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it