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Record W4415167686 · doi:10.1080/17576180.2025.2571030

Performance properties of filter-paper used in blood spot collection devices for quantitation of phenylalanine

2025· article· en· W4415167686 on OpenAlexaff
Annabel Rodham, Christopher von Ruhland, Rachel S. Carling, Stuart J. Moat

Bibliographic record

VenueBioanalysis · 2025
Typearticle
Languageen
FieldBiochemistry, Genetics and Molecular Biology
TopicMetabolism and Genetic Disorders
Canadian institutionsSt. Thomas Hospital
Fundersnot available
KeywordsPhenylalanineDried blood spotDried bloodBlood collectionWhole blood

Abstract

fetched live from OpenAlex

AIMS: Accurate and precise measurement of dried blood spot (DBS) phenylalanine (Phe) is vital for managing phenylketonuria (PKU). Standard DBS collection devices use grade-226 filter-paper, while the CapitainerB quantitative device utilizes grade-222 filter-paper. Although grade-226 filter-paper performance is well characterized, data on grade-222 filter-paper are sparse. This study aimed to investigate the analytical properties of grade-222 and grade-226 filter-papers. MATERIALS AND METHODS: We compared grade-222 and grade-226 filter-papers for Phe measurement accuracy and imprecision in DBS generated using both filter-papers. Scanning electron microscopy (SEM) and slit lamp imaging were used to assess the physical properties of the filter-papers. RESULTS: Using an aqueous calibrator as reference, grade-222 exhibited a mean bias of -1.1%, the mean bias for grade-226 was -7.3%. Intra-assay imprecision was 2.3% for grade-222, versus 4.2% for grade-226. SEM revealed that fibers in grade-226 filter-paper are bonded by an amorphous material, which is absent in grade-222 filter-paper. Total error analysis indicated grade-222 filter-paper reduced uncertainty of Phe measurement compared to grade-226 filter-paper. CONCLUSIONS: Grade-222 filter-paper was proven to have superior analytical performance for Phe quantification, providing improved differentiation between safe and harmful Phe concentrations and offering more reliable PKU monitoring compared to traditional grade-226 filter-paper.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.004
metaresearch head score (Gemma)0.010
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score0.021

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0040.010
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0020.001
Science and technology studies0.0010.001
Scholarly communication0.0020.001
Open science0.0010.001
Research integrity0.0020.000
Insufficient payload (model declined to judge)0.0020.002

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.244
Teacher spread0.231 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2025
Admission routes1
Has abstractyes

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