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Enregistrement W1589804111 · doi:10.2172/15005725

Transmutation of radioactive nuclear waste

2000· report· en· W1589804111 sur OpenAlexaboutno aff
A. H. Toor, Reiner Buck

Notice bibliographique

Revuenon disponible
Typereport
Langueen
DomaineEngineering
ThématiqueNuclear and radioactivity studies
Établissements canadiensnon disponible
Organismes subventionnairesnon disponible
Mots-clésPlutoniumTonnePlutonium-239Radioactive wasteNuclear fissionWaste managementNuclear transmutationFission productsSpent nuclear fuelPopulationPlutonium-240FissionEnvironmental scienceRadiochemistryNuclear physicsChemistryEngineeringPhysicsNeutronEnvironmental health

Résumé

récupéré en direct d'OpenAlex

Lack of a safe disposal method for radioactive nuclear waste (RNW) is a problem of staggering proportion and impact. A typical LWR fission reactor will produce the following RNW in one year: minor actinides (i.e. {sup 237}Np, {sup 242-243}Am, {sup 243-245}Cm) {approx}40 kg, long-lived fission products (i.e, {sup 99}Tc, {sup 93}Zr, {sup 129}I, {sup 135}Cs) {approx}80 kg, short lived fission products (e.g. {sup 137}Cs, {sup 90}Sr) {approx}50kg and plutonium {approx}280 kg. The total RNW produced by France and Canada amounts to hundreds of metric tonnes per year. Obtaining a uniform policy dealing with RNW has been blocked by the desire on one hand to harvest the energy stored in plutonium to benefit society and on the other hand the need to assure that the stockpile of plutonium will not be channeled into future nuclear weapons. In the meantime, the quantity and handling of these materials represents a potential health hazard to the world's population and particularly to people in the vicinity of temporary storage facilities. In the U.S., societal awareness of the hazards associated with RNW has effectively delayed development of U.S. nuclear fission reactors during the past decade. As a result the U.S. does not benefit from the large investment of resources in this industry. Reluctance to employ nuclear energy has compelled our society to rely increasingly on non-reusable alternative energy sources; coal, oil, and natural gas. That decision has compounded other unresolved global problems such as air pollution, acid rain, and global warming. Relying on these energy sources to meet our increasing energy demands has led the U.S. to increase its reliance on foreign oil; a policy that is disadvantageous to our economy and our national security. RNW can be simplistically thought of as being composed of two principal components: (1) actinides with half lives up to 10{sup 6} years and (2) the broad class of fission fragments with typical half lives of a few hundred years. One approach to the RNW storage problem has been to transmute the radioactive elements into other radioactive isotopes with much shorter half-lives. Transmutation of both RNW components using neutrons has been discussed and studied over the past four decades. Most transmutation studies have examined the feasibility of using neutron-induced reactions where the neutrons would be provided by accelerator-based spallation neutron sources, tokamak fusion reactors, sub-critical fission reactors and other novel concepts. Studies have shown that all proposed transmutation processes to treat RNW using neutron reactions are deficient or marginal at best from the point of view of energy consumption and/or cost. We suggest an alternative approach that has not been considered to date: the transmutation of RNW elements using high-energy photons or gamma rays. The photo-disintegration of RNW may provide an effective way to treat reprocessed waste; waste that has been chemically separated or the residual waste left over after neutron processing. Photo-disintegration is attractive in that any isotope can be transmuted. This approach is now potentially practical because of the development of micropole undulators (MPUs) that allow us to use small storage rings to economically generate photons with gamma-ray energies and to tune these ''gamma rays'' to the peak of the cross-section resonance for various RNW elements. Because the cross sections for all RNW nuclei have a broad peak with the maximum in the 12-18 MeV range, a single MPU could be used to treat both actinide and fission fragment components of RNW. The goal of this study is to make estimates of the reaction rates and energy efficiency of the transmutation of typical RNW elements using gamma rays to establish whether or not gamma-ray transmutation should be examined as a viable alternative solution to RNW warranting further study.

Récupéré en direct depuis OpenAlex et désinversé. Les résumés ne sont pas conservés dans cette base de données : les index inversés représentent 8,6 Go des 9,3 Go de texte de la base, et le serveur dispose de 13 Go libres.

Comment cette classification a été obtenuedéplier

Prédiction distillée sur la base complète

Imitation des enseignants

Ni prévalence calibrée, ni vérité terrain. Validation humaine à venir. Apprise à partir de 10 348 étiquettes directes de Codex et de 10 348 étiquettes directes de Gemma. Le mode candidate est l'union des têtes enseignantes seuillées; le consensus est leur intersection. Ces sorties portent le statut machine_predicted_unvalidated et ne sont ni des étiquettes humaines ni des étiquettes directes de modèles de pointe.

score de la tête « metaresearch » (Codex)0,000
score de la tête « metaresearch » (Gemma)0,000
Version: codex-gemma-dda1882f352aStatut de validation: machine_predicted_unvalidated
Catégories candidatesaucune
Catégories consensuellesaucune
DomaineSignal candidat: aucune · Signal consensuel: aucune
Devis d'étudeSignal candidat: Sans objet · Signal consensuel: Sans objet
GenreSignal candidat: Autre · Signal consensuel: aucune
Score de désaccord entre enseignants0,980
Score d'incertitude au seuil0,772

Scores Codex et Gemma par catégorie

CatégorieCodexGemma
Métarecherche0,0000,000
Méta-épidémiologie (sens strict)0,0000,000
Méta-épidémiologie (sens large)0,0000,000
Bibliométrie0,0000,000
Études des sciences et des technologies0,0000,000
Communication savante0,0000,000
Science ouverte0,0000,000
Intégrité de la recherche0,0000,000
Charge utile insuffisante (le modèle a refusé de juger)0,0010,000

Scores machine (provisoires)

Les deux têtes enseignantes du modèle étudiant, lues sur ce travail. Un score ordonne la base pour la relecture; il n'affirme jamais une catégorie, et le statut de validation accompagne chaque rangée tel quel.

Scores de référence d'un modèle non mature (critères de maturité non atteints, 7 itérations). Un score ordonne; il n'affirme jamais une catégorie.

Tête enseignante Opus0,015
Tête enseignante GPT0,227
Écart entre enseignants0,212 · la distance entre les deux têtes enseignantes sur ce seul travail
Statut de validationscore_only:v0-immature-baseline · tel quel depuis la passe de notation : score_only signifie que le nombre peut ordonner les travaux, et qu'aucune étiquette de catégorie n'en découle

Classification

machine, non validée

Prédiction automatique; un appel candidat d’une seule tête enseignante, pas un consensus.

Les modèles n’ont appliqué aucune catégorie : rien dans la taxonomie ne correspondait à ce travail.
Devis d'étudeSans objet
Domainenon disponible
GenreAutre

Le détail, modèle par modèle et score par score, se trouve en fin de page sous « Comment cette classification a été obtenue ».

En bref

Citations0
Publié2000
Routes d'admission1
Résumé présentoui

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