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Record W1491511672 · doi:10.1002/jemt.22398

Validity of the dipole approximation in TEM‐EELS studies

2014· article· en· W1491511672 on OpenAlex
R.F. Egerton, Robert A. McLeod, Marek Malac

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueMicroscopy Research and Technique · 2014
Typearticle
Languageen
FieldMaterials Science
TopicElectron and X-Ray Spectroscopy Techniques
Canadian institutionsNational Institute for NanotechnologyUniversity of Alberta
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsDipoleDiscrete dipole approximationMaterials scienceNanotechnologyPhysicsQuantum mechanics

Abstract

fetched live from OpenAlex

Nondipole effects in electron energy-loss spectroscopy are evaluated in terms of deviation of the inelastic scattering from a Lorentzian angular distribution, which is assumed in established procedures for plural-scattering deconvolution, thickness measurement, and Kramers-Kronig analysis. The deviation appears to be small and may be outweighed by the effect of plural (elastic + inelastic) scattering, which is not removed by conventional deconvolution methods. In the core-loss region of the spectrum, non-Lorentzian behaviour stems from a reduction of the generalized oscillator strength from its optical value and (for energies far above an ionization threshold) formation of a Bethe-ridge angular distribution. At incident energies above 200 keV, retardation effects further distort the angular dependence, even for core losses just above threshold. With an on-axis collection aperture, non-dipole effects are masked by the rapid falloff of intensity with scattering angle, but they may become important for off-axis measurements. Near-edge fine structure is sensitive to nondipole effects but these can be minimized by use of an angle-limiting collection aperture.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.004
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.038
Threshold uncertainty score0.331

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0040.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.061
GPT teacher head0.402
Teacher spread0.341 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it