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Record W1547676458 · doi:10.1063/1.1464831

Infrared emission spectroscopy of the [10.5]5Δ–X5Δ system of VF

2002· article· en· W1547676458 on OpenAlexaff
R. S. Ram, P. F. Bernath, Sumner P. Davis

Bibliographic record

VenueThe Journal of Chemical Physics · 2002
Typearticle
Languageen
FieldPhysics and Astronomy
TopicAdvanced Chemical Physics Studies
Canadian institutionsUniversity of Waterloo
FundersNational Aeronautics and Space AdministrationNational Science Foundation
KeywordsAnalytical Chemistry (journal)VanadiumExcited stateSpectroscopyChemistryEmission spectrumMicrowaveHeliumInfraredSpectrometerAtomic physicsSpectral linePhysicsOpticsInorganic chemistry

Abstract

fetched live from OpenAlex

The emission spectrum of VF has been investigated in the 3400–17 000 cm−1 region using a Fourier transform spectrometer. The bands were excited in a high temperature carbon tube furnace from the reaction of vanadium metal vapor with CF4, as well as in a microwave discharge through a flowing mixture of VF4 vapor and helium. Several bands observed in the 9000–12 000 cm−1 region have been attributed to VF. The bands with high wave number R heads near 9156.8, 9816.4, 10 481.4, 11 035.8, and 11 587.2 cm−1 have been assigned as the 0-2, 0-1, 0-0, 1-0, and 2-0 bands, respectively, of the new [10.5]5Δ–X5Δ system of VF. A rotational analysis of the Δ15–Δ15, Δ25–Δ25, Δ35–Δ35, and Δ45–Δ45 subbands of the 0-1, 0-0, 1-0, and 2-0 bands has been carried out and spectroscopic parameters for VF have been obtained for the first time. The following equilibrium constants have been determined for the ground state of VF by averaging the constants of the different spin components: ΔG(1/2)=665.10 cm−1, Be=0.3863 cm−1, αe=0.0028 cm−1, and re=1.7758 Å.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.096
Threshold uncertainty score0.402

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.233
Teacher spread0.222 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations19
Published2002
Admission routes1
Has abstractyes

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