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Record W1615909119 · doi:10.1029/2011gb004226

Potential role of inorganic polyphosphate in the cycling of phosphorus within the hypoxic water column of Effingham Inlet, British Columbia

2012· article· en· W1615909119 on OpenAlexaboutno aff
Julia M. Diaz, Ellery D. Ingall, Samuel D. Snow, Claudia R. Benitez‐Nelson, Martial Taillefert, Jay A. Brandes

Bibliographic record

VenueGlobal Biogeochemical Cycles · 2012
Typearticle
Languageen
FieldEnvironmental Science
TopicAquatic Ecosystems and Phytoplankton Dynamics
Canadian institutionsnot available
FundersNational Science Foundation
KeywordsWater columnRedoxEnvironmental chemistryChemistryPolyphosphatePhosphorusSaturation (graph theory)ParticulatesRemineralisationAnoxic watersPhosphateInorganic chemistryGeologyOceanographyFluoride

Abstract

fetched live from OpenAlex

The upper basin of Effingham Inlet possesses permanently anoxic bottom waters, with a water column redox transition zone typically occurring at least 40 m above the sediment‐water interface. During our sampling campaign in April and July 2007, this redox transition zone was associated with sharp peaks in a variety of parameters, including soluble reactive phosphorus (SRP) and total particulate phosphorus (TPP). Based on sequential extraction results, TPP maxima exhibited preferential accumulation of an operationally defined class of loosely adsorbed organic phosphorus (P), which may contain a substantial fraction of polyphosphate (poly‐P). This poly‐P may furthermore be involved in the redox‐dependent remobilization of SRP. For example, direct fluorometric analysis of poly‐P content revealed that particulate inorganic poly‐P was present at concentrations ranging from 1 to 9 nM P within and several meters above the TPP maximum. Below the depth of 1% oxygen saturation, however, particulate inorganic poly‐P was undetectable (<0.8 nM in situ). Assuming this concentration profile reflects the remineralization of inorganic poly‐P to SRP across the redox transition, inorganic poly‐P degradation accounted for as much as 4 ± 3% (average ± standard deviation) to 9 ± 8% of the vertical turbulent diffusive SRP flux. This finding is a conservative estimate due in part to sample storage effects associated with our analysis of poly‐P content. By comparison, iron‐linked P cycling accounted for at most 65 ± 33% of the diffusive SRP flux, leaving ∼25% unaccounted for. Thus, while redox‐sensitive poly‐P remineralization in Effingham Inlet appears modest based on our direct conservative estimate, it may be higher from a mass balance viewpoint. Poly‐P cycling may therefore be an overlooked mechanism for the redox‐sensitive cycling of P in some hypoxic/anoxic boundaries, especially iron‐poor marine oxygen minimum zones.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.241
Threshold uncertainty score0.947

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.189
Teacher spread0.185 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations41
Published2012
Admission routes1
Has abstractyes

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