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Record W1646434402 · doi:10.1063/1.3108490

Electron Compton-like quasielastic scattering from H2, D2, and HD

2009· article· en· W1646434402 on OpenAlexafffund
R. A. Bonham, Glyn Cooper, Adam P. Hitchcock

Bibliographic record

VenueThe Journal of Chemical Physics · 2009
Typearticle
Languageen
FieldPhysics and Astronomy
TopicAtomic and Molecular Physics
Canadian institutionsMcMaster UniversityBrockhouse Institute for Materials Research
FundersNatural Sciences and Engineering Research Council of CanadaCanada Research Chairs
KeywordsSpectral lineScatteringAnomaly (physics)Quasielastic scatteringLine (geometry)Compton scatteringAtomic physicsPhysicsElectronChemistryBorn approximationSpectroscopyElectron scatteringInelastic scatteringNuclear physicsOpticsX-ray Raman scatteringCondensed matter physicsQuantum mechanics

Abstract

fetched live from OpenAlex

A significant anomaly in the ratio of the cross sections for quasielastic scattering of D(2) to H(2) in a 50:50 mixture has been reported recently [Phys. Rev. Lett. 100, 043204 (2008)]. In particular, the interpretation of quasielastic scattering provided in that work predicts that the signals should be based on the elemental content and not on the molecular structure, and thus the spectrum for HD and that for the 50:50 mixture should be effectively the same, aside from minor line shape differences. In fact the signal from H in the mixture was low by 31(4)% (or that from D was correspondingly high) when compared to the signal from H in HD. Here, an attempt is made to explain this anomaly by scattering theory calculations based on the first Born and Born-Oppenheimer approximations. The relative contributions of translational, vibrational, and rotational excitations are computed for several temperatures. The computed signals are compared to the experimental spectra of HD and the 50:50 H(2)/D(2) mixture and to pure H(2) and D(2), which were reported previously. Good agreement is found for the spectral line shapes. The predicted peak positions are also found to be in good agreement with experiment except for a slight shift in the case of D(2). However the anomalous cross section ratio of D(2) to H(2) experimentally observed in the 50:50 mixture could not be explained by this approach.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.284
Threshold uncertainty score0.414

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.226
Teacher spread0.220 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations15
Published2009
Admission routes2
Has abstractyes

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