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Record W1663600328 · doi:10.1063/1.3264688

Accurate analytic potentials for Li2(X Σ1g+) and Li2(A Σ1u+) from 2 to 90 Å, and the radiative lifetime of Li(2p)

2009· article· en· W1663600328 on OpenAlexaff
Robert J. Le Roy, Nikesh S. Dattani, John A. Coxon, Amanda Ross, P. Crozet, C. Linton

Bibliographic record

VenueThe Journal of Chemical Physics · 2009
Typearticle
Languageen
FieldPhysics and Astronomy
TopicAtomic and Molecular Physics
Canadian institutionsUniversity of New BrunswickDalhousie UniversityUniversity of Waterloo
Fundersnot available
KeywordsIsotopologueRadiative transferRange (aeronautics)Adiabatic processAtomic physicsMorse potentialPhysicsChemistryMaterials scienceQuantum mechanicsMolecule

Abstract

fetched live from OpenAlex

Extensions of the recently introduced "Morse/long-range" (MLR) potential function form allow a straightforward treatment of a molecular state for which the inverse-power long-range potential changes character with internuclear separation. Use of this function in a direct-potential-fit analysis of a combination of new fluorescence data for (7,7)Li(2), (6,6)Li(2), and (6,7)Li(2) with previously reported data for the A((1)Sigma(u) (+)) and X((1)Sigma(g) (+)) states yields accurate, fully analytic potentials for both states, together with the analytic "adiabatic" Born-Oppenheimer breakdown radial correction functions which are responsible for the difference between the interaction potentials and well depths for the different isotopologues. This analysis yields accurate well depths of D(e)=8516.709(+/-0.004) and 8516.774(+/-0.004) cm(-1) and scattering lengths of 18.11(+/-0.05) and 23.84(+/-0.05) A for the ground-states of (7,7)Li(2) and (6,6)Li(2), respectively, as well as improved atomic radiative lifetimes of tau(2p)=27.1018(+/-0.0014) ns for (7)Li(2p) and 27.1024(+/-0.0014) ns for (6)Li(2p).

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.002
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.005
Threshold uncertainty score0.016

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.002
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.001
Science and technology studies0.0010.000
Scholarly communication0.0010.001
Open science0.0010.001
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0050.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.248
Teacher spread0.241 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations124
Published2009
Admission routes1
Has abstractyes

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