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Record W1872254762 · doi:10.1002/cjce.22378

Numerical simulation of hydrogen bubble growth at an electrode surface

2015· article· en· W1872254762 on OpenAlexvenueno aff
Hongbo Liu, Liangming Pan, Jian Wen

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2015
Typearticle
Languageen
FieldEngineering
TopicHeat Transfer and Boiling Studies
Canadian institutionsnot available
FundersNational Natural Science Foundation of China
KeywordsBubbleMass transferVolume of fluid methodSupersaturationMass transfer coefficientSpargingNucleationHydrogenChemistrySherwood numberBubble pointLiquid bubbleThermodynamicsAnalytical Chemistry (journal)Materials scienceMechanicsFlow (mathematics)ChromatographyTurbulencePhysical chemistryPhysics

Abstract

fetched live from OpenAlex

Abstract A single hydrogen bubble generated at an electrode surface during water electrolysis is simulated via the volume of fluid (VOF) multiphase flow model to capture the details of the interface evolution and the mass transfer that occurs at the interface. The hydrogen bubble that grows at the electrode is driven by supersaturation of the dissolved hydrogen in the liquid. Two models are used to calculate the gas‐liquid interface mass transfer coefficient. The bubble growth from experimental results agrees closely with theoretical predictions. In addition, the mass transfer of dissolved hydrogen from the electrode surface to the bulk liquid is evaluated during the bubble nucleation and growth stages. During the nucleation stage, the mass transfer coefficient is < 5.1 × 10−5 m/s. Once the bubble embryo is formed, the mass transfer greatly increases. Before the bubble releases, the mass transfer coefficient reaches 2.8 × 10−4 m/s. More detailed information about the bubble growth is presented, including bubble‐induced convection and the concentration distribution of dissolved hydrogen around the growing bubble. The results indicate that the VOF method is suitable and reliable for simulating bubble behaviour during electrolysis or other electrochemical reactions that involve gas bubble desorption.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.017
Threshold uncertainty score0.033

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0000.000
Science and technology studies0.0010.001
Scholarly communication0.0010.000
Open science0.0010.000
Research integrity0.0020.001
Insufficient payload (model declined to judge)0.0020.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.015
GPT teacher head0.206
Teacher spread0.191 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations46
Published2015
Admission routes1
Has abstractyes

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