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Record W1883095314 · doi:10.1139/cjc-2012-0356

Theoretical investigation for the designing of novel antioxidants

2012· article· en· W1883095314 on OpenAlexvenueno aff
Asif Mahmood, Muhammad Saqib, Muhammad Ali, Bilal Khalid

Bibliographic record

VenueCanadian Journal of Chemistry · 2012
Typearticle
Languageen
FieldChemistry
TopicFree Radicals and Antioxidants
Canadian institutionsnot available
Fundersnot available
KeywordsChemistryBond-dissociation energyElectronegativityEnthalpyComputational chemistryHydrogen bondDissociation (chemistry)Intramolecular forceIonization energyHeteroatomIonizationOrganic chemistryPhysical chemistryMoleculeRing (chemistry)Thermodynamics

Abstract

fetched live from OpenAlex

In this study, the antioxidant potential of salicylic acid and its derivatives was determined. O–H bond dissociation enthalpy ionization potential and spin densities were computed, which are important characteristics of antioxidants. We have designed new antioxidants on the basis of information obtained from the results of this study and a literature review. O–H bond dissociation enthalpy, ionization potential, and spin densities of designed compounds were also calculated to analyze the effect of the size of the heterocyclic ring, the electronegativity of the heteroatom, the number of hydroxyl groups, and intramolecular hydrogen bonding. The results reveal that compounds with a larger heterocyclic ring, fewer electronegative atoms, and greater number of hydroxyl groups have enhanced antioxidant activity. A comparison of bond dissociation enthalpy of designed compounds IIIA and IV with that of phenolic acid antioxidants shows that these designed compounds are potent antioxidants. From statistical analysis, it is found that for designed compounds, good correlation was found between spin density and bond dissociation enthalpy. The present theoretical investigation will provide help to understand the biological activity of salicylic acid and its derivatives for better utilization in the fields of pharmacy and the food industry. New antioxidants with better antioxidant activity can be synthesized on the basis of the results of this study.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.007
Threshold uncertainty score0.826

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.025
GPT teacher head0.234
Teacher spread0.209 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations76
Published2012
Admission routes1
Has abstractyes

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