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Record W1927856907 · doi:10.1039/c5dt02627j

Preparation of raspberry-like ZIF-8/PS composite spheres via dispersion polymerization

2015· article· en· W1927856907 on OpenAlexafffund
He Zhu, Qi Zhang, Shiping Zhu

Bibliographic record

VenueDalton Transactions · 2015
Typearticle
Languageen
FieldChemistry
TopicMetal-Organic Frameworks: Synthesis and Applications
Canadian institutionsMcMaster University
FundersNatural Sciences and Engineering Research Council of CanadaCanada Research ChairsAustralian Government
KeywordsComposite numberSPHERESMaterials scienceNanoparticleChemical engineeringDispersion polymerizationDispersion (optics)PolymerizationBlowing a raspberryMorphology (biology)StyreneParticle (ecology)NanotechnologyPolymerCopolymerComposite materialChemistry

Abstract

fetched live from OpenAlex

Raspberry-like ZIF-8/PS composite spheres are prepared via dispersion polymerization of styrene with ZIF-8 and PVP as co-stabilizers. PVP is found to be crucial in determining morphology of the final product. It helps adherence of ZIF-8 nanoparticles to PS spheres. It is found that ZIF-8 nanoparticles thus prepared are partially embedded into PS sphere surfaces, resulting in a stable raspberry-like structure. Surface coverage of ZIF-8 can reach up to ∼32%. The effects of ZIF-8 content and PVP concentration on the particle size and morphology are examined in detail with the mechanisms elucidated. The raspberry-like spheres can be used as a template to grow thick ZIF-8 layers on the PS spheres through subsequent solvothermal treatment, leading to the formation of polymer-core MOF-shell structure.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.824
Threshold uncertainty score0.997

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0030.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.015
GPT teacher head0.261
Teacher spread0.246 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations26
Published2015
Admission routes2
Has abstractyes

Explore more

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