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Properties Analysis of Spent Catalyst for Fixed-Bed Residue Hydrotreating Unit: Radial Distribution of Deposited Elements in Spent Catalyst Particles

2012· article· en· W1952497945 on OpenAlexvenueno aff
Yudong Sun, Chaohe Yang, Liu Ziyuan

Bibliographic record

VenueEnergy science and technology · 2012
Typearticle
Languageen
FieldEngineering
TopicCatalysis and Hydrodesulfurization Studies
Canadian institutionsnot available
Fundersnot available
KeywordsHydrodesulfurizationCatalysisResidue (chemistry)MetalChemical engineeringMaterials scienceSulfurChemistryMetallurgyMineralogyOrganic chemistry

Abstract

fetched live from OpenAlex

14 spent catalysts, which were sampled from a commercial residue hydrotreating unit at the end of an operation cycle, were analyzed by SEM to describe elements distributions along the radial direction of particles. Different from laboratory equipment, on the whole, V, Ni and S showed U-shaped pattern along the radial direction of spent catalysts. The catalyst bed has been penetrated by deposited metals and deposited massive metals on catalyst, so the pore size of catalyst decreased, diffusion resistance increased and reactants entered internal of the catalysts more difficultly. Most of the organometallic compounds hydrotreated and deposited on outside of the catalyst particles. It is showed that metals deposited on catalyst in forms of metal sulfides because the points of high metal content also have high sulfur contents unexceptionally. The structure of high metal deposition catalyst was destroyed obviously or massive irregular material has deposited on the external surface. It is verified by SEM that there is no any distribution law for deposited elements along the bed height. The change laws of deposited elements along the bed height and radial direction of particles were influenced by various factors in commercial residue hydrotrating. Key words : Residue hydrotreating unit; Spent catalyst; SEM

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.004

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.016
GPT teacher head0.233
Teacher spread0.218 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2012
Admission routes1
Has abstractyes

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