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Record W1956496868 · doi:10.1002/047084289x.rn00375

2,2-Dimethyl-5-[3-(diphenylstannyl) propyl]-1,3-dioxolan-4-one

2004· reference-entry· en· W1956496868 on OpenAlexaff
Jian Wang, Derrick L. J. Clive

Bibliographic record

VenueEncyclopedia of Reagents for Organic Synthesis · 2004
Typereference-entry
Languageen
FieldChemistry
TopicOrganometallic Compounds Synthesis and Characterization
Canadian institutionsUniversity of Alberta
Fundersnot available
KeywordsChemistryReagentSodium borohydrideSolubilitySilica gelOrganic chemistryNuclear chemistryCatalysis

Abstract

fetched live from OpenAlex

[410098-22-5] C20H24O3Sn (MW 431.10) InChI = 1S/C8H13O3.2C6H5.Sn.H/c1-4-5-6-7(9)11-8(2,3)10-6;2*1-2-4-6-5-3-1;;/h6H,1,4-5H2,2-3H3;2*1-5H;; InChIKey = PUVIBBRSMWZAIC-UHFFFAOYSA-N (title reagent behaves similar to Bu3SnH and Ph3SnH in standard free radical reactions,1 but the tin-containing by-products can be removed easily from the desired reaction products by mild hydrolysis under basic or acidic conditions1) Physical Data: colorless oil. Solubility: soluble in common organic solvents; usually used in benzene or toluene. Preparative Methods: 2-hydroxy-4-pentenoic acid,2 prepared from glyoxylic acid hydrate, is ketalized using 2,2-dimethoxypropane and TsOH·pyridine; the ketal is hydrostannylated by heating with an excess of triphenyltin hydride, and treatment of the resulting stannane with 1 equiv of I2,3 followed by reduction with sodium borohydride, gives the title compound. Purification: rapid flash chromatography over silica gel, using 1:4 ethyl acetate–hexane, affords the stannane as a colorless oil.1 Handling, Storage, and Precautions: the compound can be stored1 for several months in a freezer (−10 °C) in a sealed flask flushed with nitrogen, without significant decomposition, and is easily repurified, if necessary, by flash chromatography. The toxicity of this compound has not been studied and, as a precaution, work with this compound should be done in a fume hood and skin contact should be avoided.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Other · Consensus signal: none
Teacher disagreement score0.013
Threshold uncertainty score0.043

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0130.006

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.018
GPT teacher head0.233
Teacher spread0.215 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designNot applicable
Domainnot available
GenreOther

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

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Citations0
Published2004
Admission routes1
Has abstractyes

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