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Record W1963967323 · doi:10.1139/v01-198

1-Propanol hydrate by IR spectroscopy

2002· article· en· W1963967323 on OpenAlexvenueno aff
Jean-Joseph Ma×, Stéphane Daneault, Camille Chapados

Bibliographic record

VenueCanadian Journal of Chemistry · 2002
Typearticle
Languageen
FieldChemistry
TopicSpectroscopy and Chemometric Analyses
Canadian institutionsnot available
Fundersnot available
KeywordsChemistryHydrateHydrogen bondInfrared spectroscopyPropanolIntermolecular forceAqueous solutionMoleculeSpectroscopyPhysical chemistryAlcoholCrystallographyAnalytical Chemistry (journal)EthanolOrganic chemistry

Abstract

fetched live from OpenAlex

The mid-IR attenuated total reflectance (mid-IR–ATR) spectra of a series of 1-propanol and water mixtures were obtained. Factor analysis (FA) applied to spectra gave the spectra of three principal species and their abundance: pure water, pure propanol, and a 1-propanol hydrate (1:1). When compared to the pure solvents, the hydrate propanol bands were modified which indicated that the valence bonds were perturbed. The assignment of the hydrate IR bands was made by comparing them with those of pure 1-propanol and pure water. No monomer was observed which indicated that all species were associated. The simplest representation of the different associations is by groups of two on which an intermolecular bond (H-bond) can be placed. The exchange between the molecules can be represented by the following equation: (H2O···H2O) + (CH3CH2CH2OH···OHCH2CH2CH3) [Formula: see text] 2(CH3CH2CH2OH···OH2). The hydrate's formation constant (Kf) is 1.2 (±0.2). This value is less than the one expected from the association of freely moving molecules, indicating that the hydrophobic interactions of the 1-propanol aliphatic chains decrease the strength of the hydrogen bond between water and alcohol in the hydrate.Key words: IR spectroscopy, ATR spectroscopy, 1-propanol, liquid, aqueous solutions, eigenspectra, hydrate, factor analysis.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.005
Threshold uncertainty score0.015

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0050.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.211
Teacher spread0.200 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations64
Published2002
Admission routes1
Has abstractyes

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