MétaCan
Menu
Back to cohort
Record W1965537714 · doi:10.1021/jp3021936

Laboratory Study of pH at the Air–Ice Interface

2012· article· en· W1965537714 on OpenAlexafffund
Sumi N. Wren, D. J. Donaldson

Bibliographic record

VenueThe Journal of Physical Chemistry C · 2012
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicAtmospheric chemistry and aerosols
Canadian institutionsUniversity of Toronto
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsChemistryFluorescenceQuenching (fluorescence)CongelationAnalytical Chemistry (journal)AcridineChromatographyOrganic chemistryOptics

Abstract

fetched live from OpenAlex

A good understanding of pH at the air–ice interface is required in order to better understand phenomena occurring on frozen media. In this study, we used glancing-angle laser-induced fluorescence in conjunction with the surface- and pH-sensitive fluorescent dyes harmine and acridine to investigate pH at the air–ice interface. We followed changes in the surface region pH due to the freezing of water samples containing HCl, HNO 3, or NaOH. Freezing leaves the surface pH largely unchanged with respect to the prefreezing pH, indicating that protons are not strongly excluded during freezing. Exclusion of chloride to the ice surface on freezing was inferred via the enhanced quenching of the acridine fluorescence lifetime upon freezing samples containing HCl. Changes in surface pH due to the deposition of HCl(g) to frozen water surfaces were smaller than those seen on liquid surfaces, for the same acid loading.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.232
Teacher spread0.222 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations29
Published2012
Admission routes2
Has abstractyes

Explore more

Same venueThe Journal of Physical Chemistry CSame topicAtmospheric chemistry and aerosolsFrench-language works237,207