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Record W1965686717 · doi:10.1103/physrevb.81.125101

Microwave dielectric study of spin-Peierls and charge-ordering transitions in<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mrow><mml:mo>(</mml:mo><mml:mrow><mml:mtext>TMTTF</mml:mtext></mml:mrow><mml:mo>)</mml:mo></mml:mrow></mml:mrow><mml:mn>2</mml:mn></mml:msub><mml:msub><mml:mrow><mml:mtext>PF</mml:mtext></mml:mrow><mml:mn>6</mml:mn></mml:msub></mml:mrow></mml:math>salts

2010· article· lv· W1965686717 on OpenAlexaff
Alexandre Langlois, M. Poirier, C. Bourbonnais, P. Foury-Leylekian, A. Moradpour, Jean‐Paul Pouget

Bibliographic record

VenuePhysical Review B · 2010
Typearticle
Languagelv
FieldMaterials Science
TopicOrganic and Molecular Conductors Research
Canadian institutionsRegroupement Québécois sur les Matériaux de PointeUniversité de Sherbrooke
Fundersnot available
KeywordsCondensed matter physicsDielectricPhase diagramRelaxation (psychology)Charge (physics)Charge orderingSpin (aerodynamics)Phase transitionDeuteriumMaterials scienceField (mathematics)Phase (matter)PhysicsThermodynamicsQuantum mechanics

Abstract

fetched live from OpenAlex

We report a study of the 16.5 GHz dielectric function of hydrogenated and deuterated organic salts ${(\text{TMTTF})}_{2}{\text{PF}}_{6}$. The temperature behavior of the dielectric function is consistent with short-range polar order whose relaxation time decreases rapidly below the charge-ordering temperature. If this transition has more a relaxor character in the hydrogenated salt, charge ordering is strengthened in the deuterated one where the transition temperature has increased by more than thirty percent. We give the first account of anomalies in the dielectric function related to the spin-Peierls ground state revealing some interaction between both phases in their domain of coexistence in temperature. The variation of the spin-Peierls ordering temperature obtained under magnetic field completes the structure of the phase diagram at low field and are analyzed in the framework of the mean-field prediction.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.007
metaresearch head score (Gemma)0.007
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Science and technology studies, Scholarly communication, Open science, Research integrity, Insufficient payload (model declined to judge)
Consensus categoriesMeta-epidemiology (narrow), Science and technology studies, Research integrity, Insufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.851
Threshold uncertainty score0.998

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0070.007
Meta-epidemiology (narrow)0.0030.006
Meta-epidemiology (broad)0.0020.006
Bibliometrics0.0020.006
Science and technology studies0.0040.006
Scholarly communication0.0040.004
Open science0.0070.006
Research integrity0.0060.007
Insufficient payload (model declined to judge)0.7790.006

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.022
GPT teacher head0.276
Teacher spread0.254 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations12
Published2010
Admission routes1
Has abstractyes

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Same venuePhysical Review BSame topicOrganic and Molecular Conductors ResearchFrench-language works237,207