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Record W1966837023 · doi:10.1021/ie0600339

Model-Based Construction of Calcium Sulfate Phase-Transition Diagrams in the HCl−CaCl<sub>2</sub>−H<sub>2</sub>O System between 0 and 100 °C

2006· article· en· W1966837023 on OpenAlexafffund
Zhibao Li, George P. Demopoulos

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2006
Typearticle
Languageen
FieldMaterials Science
TopicCrystallization and Solubility Studies
Canadian institutionsMcGill University
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsAnhydriteMetastabilitySupersaturationPhase diagramPhase transitionHemihydrateChemistryThermodynamicsPhase (matter)ScalingCrystallographyMineralogyMaterials scienceGypsumMetallurgyPhysics

Abstract

fetched live from OpenAlex

Phase-transition diagrams of three CaSO 4 phases, namely, dihydrate, hemihydrate, and anhydrate, in the HCl−CaCl 2 −H 2 O system are successfully constructed making use of a recently developed OLI-based chemical model. After initial validation of the model by comparison to experimentally determined CaSO 4 phase-transition points in H 2 O or pure HCl solutions, the phase-transition border between dihydrate and anhydrite and that between dihydrate and hemihydrate was obtained by calculating the solution supersaturation (or scaling tendency according to OLI). The constructed phase-transition diagrams show three main regions, namely, regions I, II, and III. In region I, dihydrate is stable, while anhydrite is stable in regions II and III. Dihydrate is metastable in region II, while hemihydrate is metastable in region III. An increase in HCl and/or CaCl 2 concentration causes the metastable region of HH to expand at the expense of DH. This has the result of lowering the corresponding transition temperatures.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score0.006

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0020.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.081
GPT teacher head0.317
Teacher spread0.236 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations85
Published2006
Admission routes2
Has abstractyes

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