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Record W1968853843 · doi:10.1021/ma801398a

Phase Behavior of Ternary Homopolymer/Gradient Copolymer Blends

2009· article· en· W1968853843 on OpenAlexaff
Rui Wang, Weihua Li, Yingwu Luo, Bo‐Geng Li, An‐Chang Shi, Shiping Zhu

Bibliographic record

VenueMacromolecules · 2009
Typearticle
Languageen
FieldMaterials Science
TopicBlock Copolymer Self-Assembly
Canadian institutionsMcMaster University
Fundersnot available
KeywordsCopolymerMaterials scienceTernary operationPhase (matter)Polymer blendPolymerPolymer chemistryPhase diagramRandom phase approximationChemistryComposite materialPhysicsOrganic chemistry

Abstract

fetched live from OpenAlex

The phase behavior of ternary homopolymer/gradient copolymer blends is studied theoretically using a multiblock model of gradient copolymers. Critical lines and Lifshitz points of the blends are determined by a random phase approximation analysis. Phase diagrams and microphase structures of the blends are studied using self-consistent mean-field theory. It is discovered that the chain gradient distribution has a significant effect on the phase behavior of the blends. When the chain gradient distribution is gradual, a larger amount of copolymers and a higher incompatibility are needed for the formation of a microphase. In addition, the ability of copolymer domains to absorb homopolymers decreases, whereas the solubility of copolymers in homopolymer matrix increases, as the gradient distribution becomes gradual. Another important effect is that gradient copolymers lead to a broad interface between two incompatible polymers. These results indicate that interfacial structure and morphology of these blends can be fine-tuned by specifically designed gradient distributions.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.005

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0020.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.272
Teacher spread0.261 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations41
Published2009
Admission routes1
Has abstractyes

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