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Ionic Selectivity Inside Solid-State Nanoscale Channels: Physics and Applications

2013· article· en· W1969397989 on OpenAlexvenueno aff
Xianzu Gong, Jichen Li, Ke Xu

Bibliographic record

VenueJournal of Applied Solution Chemistry and Modeling · 2013
Typearticle
Languageen
FieldEngineering
TopicNanopore and Nanochannel Transport Studies
Canadian institutionsnot available
FundersCentro Nacional de Investigaciones CardiovascularesNational Natural Science Foundation of China
KeywordsNanoporeIonic bondingNanotechnologyIonic radiusIonChemical physicsSelectivityNanoscopic scaleSemiconductorCarbon nanotubeChemistryMaterials scienceOptoelectronicsOrganic chemistry

Abstract

fetched live from OpenAlex

Abstract: Ionic selectivity across nanochannels is of great importance to biological activities as well as for designing novel molecular devices/sensors which has wide potential applications in nanotechnology. With the development of experimental and computational facilities and technologies, it becomes possible to study the ionic selectivity inside and across the nanoscale channels by both experiments and simulations. Because of the confinement effect, there are new physical phenomena in such nanotube that are not observed at macrofluidic or microfluidic size scales, including the anomalous hydration shell order, ionic selectivity based on the surface charge. These novel properties lay the foundation for the selectivity of the various types of ions. Several controlling methods for selecting ions are designed and developed, such as a controllable ion-selective nanopore (for selecting K+ and Na+) based on a single-walled carbon nanotube with specially arranged carbonyl oxygen atoms modified inside the nanopore, which was inspired by the structure of biological ionic channels; Nanopores in graphene sheets with different functional units have been applied to sieve cations of alkali metals or anions of group 17 element, respectively; The pore radius can also be determinant factor for choosing ions. Recently, the separation of the positive and negative ions has appealed more concerns. Inside of nanofluidic nanopores, negative and positive ions are manipulated analogously to semiconductor devices such as metal-oxide-semiconductor field effect transistors, where negative and positive charged carriers are manipulated. In this review, we examine some of the recent advances in the dynamics of the ionic selectivity inside solid state nanoscale channels.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.328
Threshold uncertainty score0.501

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.217
Teacher spread0.203 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2013
Admission routes1
Has abstractyes

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