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Record W1970208107 · doi:10.1021/ef0502812

Thermogravimetric Studies on Pyrolysis and Combustion Behavior of a Heavy Oil and Its Asphaltenes

2006· article· en· W1970208107 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueEnergy & Fuels · 2006
Typearticle
Languageen
FieldChemistry
TopicPetroleum Processing and Analysis
Canadian institutionsSaskatchewan Research Council (Canada)University of Regina
FundersNatural Sciences and Engineering Research Council of CanadaPetroleum Technology Research Centre
KeywordsAsphalteneThermogravimetric analysisCokePyrolysisActivation energyArrhenius equationCombustionIsothermal processChemistryReactivity (psychology)Chemical engineeringOrganic chemistryMaterials scienceThermodynamics

Abstract

fetched live from OpenAlex

A thermogravimetric analyzer (TGA) was used to obtain information on the pyrolysis and combustion behavior of both crude oil (Neilburg) and its asphaltenes, each mixed with reservoir sand. Of all the saturate, aromatic, resin, and asphaltene fractions, asphaltenes contribute the most to the formation of coke (fuel). Temperature-ramped as well as the isothermal pyrolysis experiments on whole oil and asphaltenes were analyzed to determine the temperature at which coke formation was maximized. Furthermore, isothermal combustion curves for coke derived from whole oil and asphaltenes were obtained to provide reliable data for calculating the kinetics of the reactions. The classical Arrhenius model was applied, and the activation energy for the combustion of coke formed from pure asphaltenes and from the whole oil was calculated. The results showed that the Arrhenius model fitted the data well in the entire range of temperatures the experiments were conducted. The source material for the coke led to modest differences in its reactivity. The observed activation energy for asphaltenes was 117.7 kJ/mol, and for the whole oil it was 129.5 kJ/mol, which indicates that they were in close agreement. Also, the combustion of coke from asphaltenes showed a reaction order of 0.4 at 375°C, which gradually increased to 0.9 at 525°C. For whole oil, it increased from 0.5 at 375°C to 0.7 at 500°C.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.163
Threshold uncertainty score0.490

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.016
GPT teacher head0.255
Teacher spread0.238 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it