MétaCan
Menu
Back to cohort
Record W1972010126 · doi:10.1039/b502371h

O(1D2) orbital orientation in the ultraviolet photodissociation of ozone

2005· article· en· W1972010126 on OpenAlexaff
Suk Kyoung Lee, Dave Townsend, O. S. Vasyutinskiǐ, Arthur G. Suits

Bibliographic record

VenuePhysical Chemistry Chemical Physics · 2005
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicAtmospheric Ozone and Climate
Canadian institutionsSteacie Institute for Molecular Sciences
Fundersnot available
KeywordsPhotodissociationRecoilUltravioletAnisotropyDissociation (chemistry)Polarization (electrochemistry)ExcitationChemistryWavelengthOrientation (vector space)Atomic physicsMolecular physicsPhysicsPhotochemistryOpticsPhysical chemistry

Abstract

fetched live from OpenAlex

We present the absolute velocity-dependent orbital orientation for O(1D2) atoms produced from the photodissociation of ozone in the 248-285 nm region obtained using the DC slice imaging method. The results are analyzed in terms of laboratory frame anisotropy parameters describing distinct excitation and dissociation mechanisms possessing characteristic angular distributions. The results show negligible orbital orientation produced in dissociation by circularly polarized light, but strong recoil speed-dependent orientation following photolysis by linearly polarized light at all wavelengths studied. The origin of this polarization is ascribed to nonadiabatic transitions at avoided crossings and at long range.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.046
Threshold uncertainty score0.386

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.225
Teacher spread0.217 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations43
Published2005
Admission routes1
Has abstractyes

Explore more

Same venuePhysical Chemistry Chemical PhysicsSame topicAtmospheric Ozone and ClimateFrench-language works237,207