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Record W1974523190 · doi:10.1021/ef049956b

Methodology for the Characterization and Modeling of Asphaltene Precipitation from Heavy Oils Diluted with <i>n</i>-Alkanes

2004· article· en· W1974523190 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.
aboutThe title or abstract carries a Canadian signal from the geographic lexicon.

Bibliographic record

VenueEnergy & Fuels · 2004
Typearticle
Languageen
FieldChemistry
TopicPetroleum Processing and Analysis
Canadian institutionsUniversity of Calgary
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsAsphalteneMolar massSolubilityTolueneChemistryPrecipitationHildebrand solubility parameterFraction (chemistry)HeptaneMolar volumeAlkaneMole fractionChromatographyAnalytical Chemistry (journal)HydrocarbonOrganic chemistryThermodynamicsPhysical chemistryPolymer

Abstract

fetched live from OpenAlex

A regular solution model, previously used to model asphaltene precipitation from Western Canadian bitumens, was tested on four international heavy oil and bitumen samples. The input parameters for the model are the mole fraction, the molar volume, and the solubility parameter for each component. Heavy oils and bitumens were divided into four main pseudo-components, corresponding to the SARA fractions (saturates, aromatics, resins, and asphaltenes). Asphaltenes were divided into fractions of different molar mass, based on a gamma molar mass distribution. The molar volumes and solubility parameters of the pseudo-components were calculated using solubility, density, and molar mass measurements and previously developed correlations. Model predictions were compared with the measured onset and the amount of asphaltene precipitation for solutions of asphaltenes in toluene and n -heptane and for heavy oils diluted with n -alkanes, all under ambient conditions. The overall average absolute deviations (AAD) of the predicted fractional precipitation or yields were <0.031 for the asphaltene solutions and <0.008 for the diluted heavy oils. A methodology for characterizing heavy oils and modeling asphaltene precipitation from n -alkane-diluted heavy oils is proposed.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.406
Threshold uncertainty score0.283

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.033
GPT teacher head0.264
Teacher spread0.231 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it