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Record W1975645876 · doi:10.1021/ef700786u

Interfacial Films Adsorbed from Bitumen in Toluene Solution at a Toluene−Water Interface: A Langmuir and Langmuir−Blodgett Film Approach

2008· article· en· W1975645876 on OpenAlexafffund
M. Sharath Chandra, Zhenghe Xu, Jacob H. Masliyah

Bibliographic record

VenueEnergy & Fuels · 2008
Typearticle
Languageen
FieldChemistry
TopicPetroleum Processing and Analysis
Canadian institutionsUniversity of Alberta
FundersNatural Sciences and Engineering Research Council of CanadaSyncrude
KeywordsTolueneLangmuirAsphalteneAdsorptionLangmuir–Blodgett filmChemical engineeringLangmuir adsorption modelPhase (matter)AsphaltMaterials scienceChemistryOrganic chemistryMoleculeComposite material

Abstract

fetched live from OpenAlex

Using Langmuir and Langmuir−Blodgett (LB) film techniques, the present study shows that interfacial film formation is due to the adsorption of bituminous compounds at a toluene−water interface. Langmuir films formed using various concentrations of the bituminous compounds below their critical micelle concentration or critical nanoaggregate concentration in the toluene phase indicate that asphaltenes, a constituent of bitumen, irreversibly adsorb at the toluene−water interface. Based on Langmuir and LB film studies, the pressure−area isotherms as well as the morphology, thickness, and the hydrophobicity of the interfacial films are similar when bitumen and asphaltenes were independently used as the source for the surface active materials present in the bulk organic phase. Morphology and thickness studies on the corresponding LB films suggest the formation of discoid nanoaggregates with a definite size at the interface.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.028
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.218
Teacher spread0.205 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations24
Published2008
Admission routes2
Has abstractyes

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