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Record W1977183960 · doi:10.1021/ma0021592

Wettability of Maleimide Copolymer Films:  Effect of the Chain Length of <i>n</i>-Alkyl Side Groups on the Solid Surface Tension

2001· article· en· W1977183960 on OpenAlex
Karina Grundke, Stefan Zschoche, Kathrin Pöschel, Thomas Gietzelt, Stefan Michel, Peter Friedel, Dieter Jehnichen, A. W. Neumann

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueMacromolecules · 2001
Typearticle
Languageen
FieldChemistry
TopicSurfactants and Colloidal Systems
Canadian institutionsUniversity of Toronto
Fundersnot available
KeywordsSide chainAlkylCopolymerPolymer chemistryMaleimideChemistryStyreneSurface tensionContact angleWettingSurface energyMaterials scienceOrganic chemistryPolymerComposite materialPhysical chemistry

Abstract

fetched live from OpenAlex

We report bulk and surface properties of maleimide copolymers with two different backbones, poly(propene- alt - N -( n -alkyl)maleimides) (PAlkMI) and poly(styrene- alt - N -( n -alkyl) maleimides) (SAlkMI), with different lengths of n -alkyl side chains (methyl, ethyl, propyl, butyl, pentyl, hexyl, octyl, and dodecyl). The contact angle and solid surface tension results suggest that, for the longer side chains, the surface properties are dominated by the side chains. Indeed, the surface tension of the two types of copolymers with length of the side chain above C = 6 are essentially equal, indicating complete shielding of the polar backbone chain. For the two copolymers containing dodecyl side chains, the solid surface tension is similar to that of solid surfaces consisting exclusively of CH 3 groups. Apparently, these side groups are long enough to allow arrangement in the configuration of the lowest surface free energy possible for alkyl chains. For the short side chain copolymers the styrene compounds are more hydrophobic than the propene compounds. The bulkier phenyl rings shields the polar backbone chain more effectively than the small alkyl groups.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.026
Threshold uncertainty score0.543

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.224
Teacher spread0.216 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it