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Record W1977986458 · doi:10.1039/c0cc03463k

Cationic zinc complexes: a new class of catalyst for living lactide polymerization at ambient temperature

2010· article· en· W1977986458 on OpenAlex
Craig A. Wheaton, Paul G. Hayes

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueChemical Communications · 2010
Typearticle
Languageen
FieldMaterials Science
Topicbiodegradable polymer synthesis and properties
Canadian institutionsUniversity of Lethbridge
Fundersnot available
KeywordsCationic polymerizationPolymerizationCatalysisLactideZincPolymer chemistryChemistryPincer movementPincer ligandLigand (biochemistry)Living cationic polymerizationKineticsRing-opening polymerizationCoordination polymerizationPolymerOrganic chemistrySolution polymerization

Abstract

fetched live from OpenAlex

Cationic zinc complexes of a bis(phosphinimine) pincer ligand have been prepared. Methylzinc and zinc-lactate complexes have been structurally characterized, and the latter is the first cationic metal complex to promote coordination-insertion polymerization of lactide at ambient temperature. This novel catalyst system is remarkably active and also exhibits living character. A detailed investigation of the kinetics and mechanism of the polymerization process has been undertaken.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.010
Threshold uncertainty score0.429

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.032
GPT teacher head0.264
Teacher spread0.232 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it