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Record W1978534706 · doi:10.1002/bip.20416

Intercalation of daunomycin into d(CG)<sub>4</sub> oligomer duplex containing G·T mismatches by vibrational circular dichroism and infrared absorption spectroscopy

2005· article· en· W1978534706 on OpenAlexaff
Aleksandra A. Pandyra, D. Tsankov, Valery Andrushchenko, J.H. van de Sande, H. Wieser

Bibliographic record

VenueBiopolymers · 2005
Typearticle
Languageen
FieldBiochemistry, Genetics and Molecular Biology
TopicDNA and Nucleic Acid Chemistry
Canadian institutionsUniversity of Calgary
Fundersnot available
KeywordsChemistryVibrational circular dichroismInfrared spectroscopyHistone octamerCrystallographyCircular dichroismAbsorption (acoustics)InfraredSpectroscopyIntercalation (chemistry)StereochemistryDNAOpticsOrganic chemistry

Abstract

fetched live from OpenAlex

Abstract The vibrational circular dichroism (VCD) and infrared absorption (IR) spectra of the mismatched octamer oligonucleotides d(CGTGCGCG) 2 ( CGT ) and d(CGCGTGCG) 2 ( CGC ) and their complexes with the antitumor drug daunomycin were measured in D 2 O, interpreted, and compared to the octamer d(CGCGCGCG) 2 ( CG ). The IR spectra of the mismatched octamers in the carbonyl‐stretching region are similar to those of the parent CG, whereas the VCD spectra differ in several respects between each other. The main VCD feature due to carbonyl stretching is informative for the mismatches and CG . Vibrational modes in the sugar–phosphate region remain essentially unchanged especially for PO 2 − symmetric stretching. Differences between the free and complexed mismatch octamers occurred mainly in the carbonyl‐stretching region (1700–1600 cm −1 ). The absorption intensity of the CO peak of G is more prominent for CGC than CGT and resembles CG in this respect. The detailed composition of this doublet is clearly visible, indicating the geometric rearrangement of the base pairs in the presence of the mismatch and upon forming the daunomycin complex. © 2005 Wiley Periodicals, Inc. Biopolymers 82: 189–198, 2006 This article was originally published online as an accepted preprint. The “Published Online” date corresponds to the preprint version. You can request a copy of the preprint by emailing the Biopolymers editorial office at biopolymers@wiley.com

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score0.740

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.212
Teacher spread0.208 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2005
Admission routes1
Has abstractyes

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