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Record W1979682283 · doi:10.1088/0953-4075/40/1/011

Ultrafast imaging of multielectronic dissociative ionization of CO<sub>2</sub>in an intense laser field

2006· article· en· W1979682283 on OpenAlexafffund
J.-P. Brichta, Spencer Walker, R Helsten, J H Sanderson

Bibliographic record

VenueJournal of Physics B Atomic Molecular and Optical Physics · 2006
Typearticle
Languageen
FieldPhysics and Astronomy
TopicLaser-Matter Interactions and Applications
Canadian institutionsUniversity of Waterloo
FundersGovernment of Ontario
KeywordsPhysicsCoulomb explosionAtomic physicsIonizationExcited stateIonLaserKinetic energyPolyatomic ionDouble ionizationMomentum (technical analysis)MoleculeSpectral lineField (mathematics)OpticsQuantum mechanics

Abstract

fetched live from OpenAlex

Momentum vectors of fragment ions produced by the Coulomb explosion of CO2z+ (z = 3–6) in an intense laser field (∼50 fs, 1 × 1015 W cm−2) are determined by the triple coincidence imaging technique. The molecular structure from symmetric and asymmetric explosion channels is reconstructed from the measured momentum vectors. The channel-dependent mean C–O bond length of ⟨r⟩ = 2.14–3.89 Å and the O–C–O bend angle of ⟨θ⟩ = 170–175° confirm substantial deformation of the molecular skeleton during the laser-molecule interaction. The channel-dependent bond length data are qualitatively described using a classical enhanced ionization model. The kinetic energy spectra reveal interesting structure which is attributed to the existence of excited states in the fragment ions.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.157
Threshold uncertainty score0.487

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.245
Teacher spread0.241 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations42
Published2006
Admission routes2
Has abstractyes

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