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Record W1980391841 · doi:10.1063/1.1362296

Monte Carlo and numerical self-consistent field study of systems with end-grafted and free polymers in good solvent

2001· article· en· W1980391841 on OpenAlexafffund
M. P. Pépin, M. D. Whitmore

Bibliographic record

VenueThe Journal of Chemical Physics · 2001
Typearticle
Languageen
FieldMaterials Science
TopicPolymer Surface Interaction Studies
Canadian institutionsMemorial University of Newfoundland
FundersNatural Sciences and Engineering Research Council of CanadaUniversité de Montréal
KeywordsMonte Carlo methodPolymerScalingPenetration (warfare)Materials scienceStatistical physicsPenetration depthContext (archaeology)SolventChemical physicsThermodynamicsPolymer chemistryPhysicsChemistryMathematicsOpticsComposite materialStatisticsOrganic chemistry

Abstract

fetched live from OpenAlex

We present a systematic Monte Carlo and numerical self-consistent field (NSCF) study of thin films consisting of grafted and free polymers in good solvent, for the range of densities found in most experiments. Above the overlap threshold for the grafted polymer, the two approaches agree well. Even at low densities, the agreement is surprisingly good. The NSCF results are also directly compared with experiments. The systematic results are interpreted in the context of the regimes and behavior predicted by scaling and analytic SCF theories. We find that the grafted layer is generally thinner, and the penetration of the free polymer into the grafted layer is generally greater than predicted, and that the overall behavior is not in accord with the earlier theories. We find it useful to introduce and distinguish between two measures of the penetration, and we find that one of them can increase with the concentration of grafted polymer.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.020
Threshold uncertainty score0.262

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.242
Teacher spread0.229 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations17
Published2001
Admission routes2
Has abstractyes

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