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Record W1982282705 · doi:10.1021/ma010108e

α-Relaxation in PEO−LiTFSI Polymer Electrolytes

2001· article· en· W1982282705 on OpenAlexaff
Guomin Mao, Marie‐Louise Saboungi, David L. Price, Michel Armand, F. Mezei, Stéphanie Pouget

Bibliographic record

VenueMacromolecules · 2001
Typearticle
Languageen
FieldEngineering
TopicAdvanced Battery Materials and Technologies
Canadian institutionsUniversité de Montréal
Fundersnot available
KeywordsElectrolyteRelaxation (psychology)PolymerChemistryDeuteriumLithium (medication)IonChemical physicsPolymer chemistryThermodynamicsMaterials sciencePhysical chemistryOrganic chemistryPhysics

Abstract

fetched live from OpenAlex

Relaxation processes in the ns time regime in deuterated pure PEO and two different concentrations of PEO−LiTFSI electrolytes show a stretched exponential behavior identifiable with translational motions of the chain segments. The time scale of the dynamics is slowed by factors of 3 and 10 as a result of adding lithium salt at EO:Li concentrations of 7.5 and 3, respectively, presumably due to the increased rigidity of the lattice caused by inter- and intrachain cross-linking by the Li ions. At the same time the stretching parameter is reduced by 35% and 50%, respectively. Measurements of the Q dependence show that both the relaxation time and the stretching parameter have a positive correlation with S ( Q ).

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.020
Threshold uncertainty score0.422

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.200
Teacher spread0.195 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations49
Published2001
Admission routes1
Has abstractyes

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