MétaCan
Menu
Back to cohort
Record W1984338301 · doi:10.1021/cm048587u

Cross-Linkable Highly Fluorinated Poly(Arylene Ether Ketones/Sulfones) for Optical Waveguiding Applications

2005· article· en· W1984338301 on OpenAlexaff
Yinghua Qi, Jianfu Ding, Michael Day, Jia Jiang, Claire L. Callender

Bibliographic record

VenueChemistry of Materials · 2005
Typearticle
Languageen
FieldMaterials Science
TopicSynthesis and properties of polymers
Canadian institutionsNational Research Council CanadaCommunications Research Centre Canada
Fundersnot available
KeywordsAryleneMaterials sciencePolymerEtherPolymer chemistryGlass transitionMonomerThermal stabilityChemical engineeringComposite materialOrganic chemistryArylAlkylChemistry

Abstract

fetched live from OpenAlex

Novel cross-linkable, highly fluorinated poly(arylene ether ketones/sulfones) have been prepared by copolycondensation reactions of perfluorinated aromatic ketone/sulfone with 4,4‘-(hexafluoroisopropylidene)diphenol and a tetrafluorostyrol-containing bisphenol (i.e., 1,1-bis(4-hydroxyphenyl)ethyl-1-phenyl 2,3,5,6-tetrafluorostyrol ether). The reactions were conducted at low temperature in the presence of calcium hydride and cesium fluoride. The resulting polymers have number-average molecular weights in the range of 25 000−36 000, excellent solubilities in common organic solvents, high glass transition temperatures ( T g ) in the region of 150−185 °C, and good thermal stabilities ( T d up to 480 °C). Tough, flexible, and transparent thin films of these polymers can be readily prepared by both solution casting and spin-coating. By adjusting the feed ratio of monomers, the refractive index and cross-linking density of the polymers can be readily controlled. Cross-linking of these polymers has been demonstrated by both thermal heating and UV irradiation. The cross-linked polymer thin films exhibit low optical loss (∼0.5 dB/cm) and low birefringence (∼2 × 10 - 3 ) at 1550 nm, demonstrating that they are promising candidates for optical waveguide materials.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.004

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.021
GPT teacher head0.275
Teacher spread0.253 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations80
Published2005
Admission routes1
Has abstractyes

Explore more

Same venueChemistry of MaterialsSame topicSynthesis and properties of polymersFrench-language works237,207