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Record W1987088543 · doi:10.1021/sc300176r

Green Chemistry of Zein Protein Toward the Synthesis of Bioconjugated Nanoparticles: Understanding Unfolding, Fusogenic Behavior, and Hemolysis

2013· article· en· W1987088543 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueACS Sustainable Chemistry & Engineering · 2013
Typearticle
Languageen
FieldMaterials Science
TopicPolymer Surface Interaction Studies
Canadian institutionsWilfrid Laurier UniversityCollege of the North Atlantic
Fundersnot available
KeywordsChemistryNucleationNanoparticleSurface plasmon resonanceAdsorptionAqueous solutionChemical engineeringAbsorbanceNanotechnologyMaterials scienceOrganic chemistryChromatography

Abstract

fetched live from OpenAlex

Green chemistry of industrially important zein protein was explored in aqueous phase toward the synthesis of bioconjugated gold (Au) nanoparticles (NPs), which allowed us to simultaneously understand the unfolding behavior of zein with respect to temperature and time. Synthesis of Au NPs was monitored with simultaneous measurements of UV–visible absorbance due to the surface plasmon resonance (SPR) of Au NPs that triggered the adsorption of zein on the NP surface and thus resulted in its unfolding. Surface adsorption of zein further controlled the crystal growth of Au NPs, which relied on the degree of unfolding and fusogenic behavior of zein due to its predominant hydrophobic nature. The latter property induced a marked blue shift in the SPR rarely observed in the growing NPs during the nucleation process. A greater unfolding of zein in fact was instrumental in generating zein-coated faceted NPs that were subjected to their hemolytic response for their possible use as drug release vehicles. Zein coating significantly reduced the hemolysis and made bioconjugated Au NPs the best models for biomedical applications in nanotechnology.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.010
Threshold uncertainty score0.803

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.213
Teacher spread0.200 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it