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Record W1988321510 · doi:10.1021/ef100884b

To Cyclopropanate or Not To Cyclopropanate? A Look at the Effect of Cyclopropanation on the Performance of Biofuels

2010· article· en· W1988321510 on OpenAlexaff
Alexandre Langlois, Olivier Lebel

Bibliographic record

VenueEnergy & Fuels · 2010
Typearticle
Languageen
FieldEngineering
TopicBiodiesel Production and Applications
Canadian institutionsRoyal Military College of Canada
Fundersnot available
KeywordsCyclopropanationChemistryAutoxidationOrganic chemistryCyclopropaneCanolaViscosityBiofuelLimoneneCatalysisThermodynamicsFood science

Abstract

fetched live from OpenAlex

The cyclopropanated derivatives of three diesel-compatible biofuels—limonene, turpentine, and canola oil methyl ester—were prepared. Their heats of combustion were both calculated using theoretical methods and measured experimentally, and it was found that for all three compounds the specific energy (in kJ/g) was similar to that of the starting materials, while the energy density (in kJ/mL) was 3−4% higher, which is slightly lower than that for the predicted values. For canola oil methyl ester, the effect of cyclopropanation on the accelerated oxidation stability was also studied, and similar trends in viscosity were observed for both the starting material and the cyclopropanated product, while no degradation of the cyclopropane groups was observed and only residual alkene groups had shown any sign of reaction, hinting that the increase in the viscosity observed with unsaturated fatty esters upon oxidation may not be directly related to autoxidation of the fatty acid chains.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.051
Threshold uncertainty score0.500

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.221
Teacher spread0.214 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations12
Published2010
Admission routes1
Has abstractyes

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