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Landau model for the elastic properties of the ferroelastic crystal Rb<sub>4</sub>LiH<sub>3</sub>(SO<sub>4</sub>)<sub>4</sub>

2009· article· en· W1995040618 on OpenAlexaff
G. Quirion, Weimin Wu, Oktay Aktas, J.L. Rideout, M. J. Clouter, B. Mróz

Bibliographic record

VenueJournal of Physics Condensed Matter · 2009
Typearticle
Languageen
FieldMaterials Science
TopicSolid-state spectroscopy and crystallography
Canadian institutionsUniversity of TorontoMemorial University of Newfoundland
Fundersnot available
KeywordsSofteningCondensed matter physicsWork (physics)Soft modesRaman scatteringCoupling (piping)ScatteringTransition temperatureThermodynamicsRaman spectroscopyMaterials scienceChemistryPhysicsOpticsQuantum mechanics

Abstract

fetched live from OpenAlex

Using sound velocity measurements, we report a detailed investigation of the elastic properties of Rb(4)LiH(3)(SO(4))(4) realized as a function of temperature and pressure. Results are compared to predictions of a phenomenological Landau model. Supported by recent Raman scattering measurements, we assume that the [Formula: see text] structural transformation observed at T(c) = 134 K corresponds to a pseudo-proper ferroelastic transition. For the numerical analysis, all coupling parameters are determined using the temperature dependence of the frequency of the soft optical B mode, the temperature dependence of spontaneous strains, and the pressure dependence dT(c)/dP = 191 ± 2 K GPa(-1) also determined in this work. Our comparison indicates that the [Formula: see text] structural transition in Rb(4)LiH(3)(SO(4))(4) is fully consistent with predictions derived using our pseudo-proper ferroelastic model. Thus, all data presented in this paper corroborate that the mechanism leading to the structural transition at T(c) = 134 K results from the softening of the B optical mode observed at 31 cm(-1). This detailed analysis also refutes the idea that Rb(4)LiH(3)(SO(4))(4) shows incomplete softening of the soft acoustic mode also associated with that structural transition.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.006
Threshold uncertainty score0.020

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.000
Science and technology studies0.0000.001
Scholarly communication0.0000.001
Open science0.0020.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0060.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.015
GPT teacher head0.226
Teacher spread0.211 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2009
Admission routes1
Has abstractyes

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