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Record W1996079205 · doi:10.1021/jp9013477

Structural Investigation of MFe<sub>2</sub>O<sub>4</sub> (M = Fe, Co) Magnetic Fluids

2009· article· en· W1996079205 on OpenAlexaff
Guilherme V. M. Jacintho, Alexandre G. Brolo, Paola Cório, Paulo A. Z. Suarez, Joel C. Rubim

Bibliographic record

VenueThe Journal of Physical Chemistry C · 2009
Typearticle
Languageen
FieldMaterials Science
TopicMagnetic Properties and Synthesis of Ferrites
Canadian institutionsUniversity of Victoria
Fundersnot available
KeywordsRaman spectroscopyAnalytical Chemistry (journal)Fourier transform infrared spectroscopyMaterials scienceAdsorptionCoprecipitationChemistryInorganic chemistryChemical engineeringPhysical chemistryOptics

Abstract

fetched live from OpenAlex

Ferrites of the type M II Fe 2 O 4 (M = Fe and Co) have been prepared by the traditional coprecipitation method. These ferrites were modified by the adsorption of fatty acids derived from soybean and castor oil and were then dispersed in cyclohexane, providing very stable magnetic fluids, readily usable in nonpolar media. The structural properties of the ferrites and modified ferrites as well as the magnetic fluids were characterized by XRD (X-ray powder diffraction), TEM (transmission electron microscopy), DRIFTS (diffusion reflectance infrared Fourier transform spectroscopy), FTNIR (Fourier transform near-infrared), UV−vis, normal Raman spectroscopy, and surface-enhanced Raman scattering (SERS). XRD and TEM analysis have shown that the magnetic nanoparticles (nonmodified and modified) present diameters in the range of 10−15 nm. DRIFTS measurements have shown that the carboxylate groups of soybean and castor oil fatty acids adsorb on the ferrite surface, forming three different structures: a bridging bidentate, a bridging monodentate, and a bidentate chelate structure. The FTIR and Raman spectra of nonmodified Fe 3 O 4 and CoFe 2 O 4 nanoparticles have shown that the number of observed phonons is not compatible with the expected O h 7 symmetry, since IR-only active phonons were observed in the Raman spectra and vice versa. SERS measurements of a CoFe 2 O 4 thin film on a SERS-active gold electrode at different applied potentials made possible the assignment of the signals near 550 and 630 cm −1 to Co−O motions and the signals near 470 and 680 cm −1 to Fe−O motions.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.217
Teacher spread0.206 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations226
Published2009
Admission routes1
Has abstractyes

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Same venueThe Journal of Physical Chemistry CSame topicMagnetic Properties and Synthesis of FerritesFrench-language works237,207