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Record W1998916250 · doi:10.1007/s11746-009-1515-z

Structured and Specialty Lipids in Continuous Packed Column Reactors: Comparison of Production Using One and Two Enzyme Beds

2009· article· en· W1998916250 on OpenAlexafffund
Fayez� Hamam, Suzanne M. Budge

Bibliographic record

VenueJournal of the American Oil Chemists Society · 2009
Typearticle
Languageen
FieldBiochemistry, Genetics and Molecular Biology
TopicEnzyme Catalysis and Immobilization
Canadian institutionsDalhousie University
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsSubstrate (aquarium)ChemistryYield (engineering)ChromatographyVolumetric flow rateResponse surface methodologyPacked bedRhizomucor mieheiAnalytical Chemistry (journal)Materials scienceBiochemistryLipaseEnzymeTriacylglycerol lipaseThermodynamicsComposite material

Abstract

fetched live from OpenAlex

Abstract In this study, speciality lipids based on fish oil (FO) and capric acid (CA) were produced in packed bed bioreactors using immobilized Lipozyme IM from Rhizomucor miehei in a solvent‐free environment. Our goal was to compare the product quality and yield among reactors consisting of one or two enzyme columns. Response surface methodology (RSM) was used to optimize process variables for maximum incorporation (Inc) of CA for each reactor configuration. The studied process variables were substrate molar ratio (1:1–3:1 CA/FO), temperature (35–55 °C) and flow rate (0.5–1.5 mL/min). All experiments were conducted based on a face‐centered cube design. The maximum predicted Inc of CA into FO (31.7 mol%) using one column was obtained when substrate molar ratio, temperature and flow rate of substrates were 2.70:1 (CA/FO), 55 °C and 0.5 mL/min. The corresponding optimal Inc of CA into FO (22.7 mol%) using two columns was predicted at 2.95:1 (CA/FO), 55 °C and 0.86 mL/min. Analysis of variance (ANOVA) showed that Inc of CA into the one‐bed design was significantly influenced by all experimental conditions, with substrate molar ratio having the greatest impact. In the two‐bed design, only temperature and flow rate had an effect; the molar ratio of substrates was not significant. Coefficients of determination were low for both designs, indicating a poor fit of our data to the model. However, the main purpose of this study was to assess the effect of process factors on Inc of CA into FO, rather than generate a model useful for prediction of responses under conditions not examined with this design. Therefore, the significant ANOVA results are much more important, stressing the real relationship between parameters and response, than the low coefficients of determination.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.010
Threshold uncertainty score0.314

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.281
Teacher spread0.269 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations20
Published2009
Admission routes2
Has abstractyes

Explore more

Same venueJournal of the American Oil Chemists SocietySame topicEnzyme Catalysis and ImmobilizationFrench-language works237,207