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Record W2001260872 · doi:10.1139/p00-087

Trends in the alkaline-earth amide series: The millimetre-wave spectrum of MgNH<sub>2</sub> and MgND<sub>2</sub> (<sup>2</sup>A<sub>1</sub>)

2001· article· en· W2001260872 on OpenAlexvenueno aff
P. M. Sheridan, L. M. Ziurys

Bibliographic record

VenueCanadian Journal of Physics · 2001
Typearticle
Languageen
FieldChemistry
TopicMolecular Spectroscopy and Structure
Canadian institutionsnot available
FundersDivision of ChemistryNational Aeronautics and Space AdministrationNational Science Foundation
KeywordsStrontiumPhysicsMoleculeIsotopomersAmideAtomic physicsSpectral lineAlkaline earth metalMagnesiumCrystallographyAnalytical Chemistry (journal)ChemistryAlkali metal

Abstract

fetched live from OpenAlex

The pure rotational spectra of MgNH 2 ([Formula: see text] 2 A 1 ) and its deuterium isotopomer have been recorded using millimetre/sub-millimetre wave direct absorption techniques. Both species were synthesized by the reaction of magnesium vapor and either NH 3 or ND 3 in a dc discharge. Twelve rotational transitions were measured for MgNH 2 , and eight transitions were observed for MgND 2 , both in the range 120–530 GHz. Asymmetry components with K a = 0–5,7, and sometimes 6, were measured for nearly every transition. Rotational, centrifugal distortion, and spin–rotation parameters have been accurately determined for both molecules, as well as an r 0 structure for magnesium amide. The data indicate that MgNH 2 is a planar molecule with C 2v symmetry, similar to CaNH 2 and SrNH 2 , and does not undergo inversion. However, there appears to be subtle differences between MgNH 2 and its calcium and strontium analogs. Magnesium amide, for example, has a significantly larger H–N–H bond angle than CaNH 2 and SrNH 2 . In addition, the spin–rotation constants indicate slightly more in-plane p character for the unpaired electron in this molecule relative to that in calcium or strontium amide. Such differences may result from more covalent character in the bonding of MgNH 2 in comparison to the heavier alkaline-earth amide species. PACS No.: 32.20Bx

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.024
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.001
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.002
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.205
Teacher spread0.196 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations4
Published2001
Admission routes1
Has abstractyes

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