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Record W2006404749 · doi:10.1103/physrevb.84.075203

Thermoelectric properties of<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mi>p</mml:mi></mml:math>-type CuInSe<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:msub><mml:mrow/><mml:mn>2</mml:mn></mml:msub></mml:math>chalcopyrites enhanced by introduction of manganese

2011· article· lv· W2006404749 on OpenAlexaff
Jinlei Yao, Nathan J. Takas, Megan L. Schliefert, David S. Paprocki, Peter E. R. Blanchard, Huiyang Gou, Arthur Mar, Christopher L. Exstrom, Scott A. Darveau, Pierre F. P. Poudeu, Jennifer A. Aitken

Bibliographic record

VenuePhysical Review B · 2011
Typearticle
Languagelv
FieldEngineering
TopicChalcogenide Semiconductor Thin Films
Canadian institutionsUniversity of Alberta
FundersU.S. Department of Energy
KeywordsThermoelectric effectSeebeck coefficientRaman spectroscopyMaterials scienceX-ray photoelectron spectroscopySemiconductorThermoelectric materialsSpectroscopyCondensed matter physicsAnalytical Chemistry (journal)PhysicsOptoelectronicsThermodynamicsChemistryNuclear magnetic resonanceOpticsQuantum mechanics

Abstract

fetched live from OpenAlex

Thermoelectric properties, x-ray photoelectron spectroscopy, Raman spectroscopy, and electronic structures have been studied for Mn-substituted CuInSe${}_{2}$ chalcopyrites. Raman spectroscopy verifies the lattice disorder due to the introduction of Mn into the CuInSe${}_{2}$ matrix, leading to a slight suppression of thermal conductivity. On the other hand, the Mn substitution significantly increases the electrical conductivity and Seebeck coefficient. Therefore the thermoelectric figure of merit $ZT$ has been enhanced by over two orders of magnitude by the introduction of Mn into CuInSe${}_{2}$. These materials are $p$-type degenerate semiconductors, containing divalent Mn species as confirmed by x-ray photoelectron spectroscopy. The crystal structure of Mn-substituted CuInSe${}_{2}$, as well as related ternary and quaternary diamond-like semiconductors, can be viewed as a combination of an electrically conducting unit, the Cu-Se and Mn-Se networks, and an electrically insulating unit, the In-Se network. Therefore, diamond-like semiconductors can serve as a potential class of thermoelectric materials with relatively wide band gaps upon substitution with Mn or other transition metals.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score0.009

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0030.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.023
GPT teacher head0.243
Teacher spread0.220 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations65
Published2011
Admission routes1
Has abstractyes

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Same venuePhysical Review BSame topicChalcogenide Semiconductor Thin FilmsFrench-language works237,207