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The Solid State 13C NMR Study of Gamma Radiation of Ethylene-Octene Copolymer

2014· article· en· W2008030103 on OpenAlex
Shaojin Jia, Zhenqi Zhang, Xiaotian Hou, Tao He, Pingkai Jiang

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

venuePublished in a venue whose home country is Canada.
no affNo Canadian affiliation: this work is invisible to an affiliation-only frame.
No Canadian affiliation. An affiliation-only frame, the usual design, would never have seen this work. It is one of the works that make the case for inverting the frame.

Bibliographic record

VenueJournal of Research Updates in Polymer Science · 2014
Typearticle
Languageen
FieldMaterials Science
TopicPolymer Nanocomposite Synthesis and Irradiation
Canadian institutionsnot available
Fundersnot available
KeywordsOcteneMaterials scienceCopolymerEthyleneCarbon-13 NMRIrradiationRadiationChain scissionSolid-state nuclear magnetic resonanceNuclear magnetic resonanceAnalytical Chemistry (journal)PolymerChemistryOrganic chemistryNuclear physicsCatalysisComposite materialPhysics

Abstract

fetched live from OpenAlex

Ethylene-octene copolymer (POE) samples exposed to γ-radiation under a series of absorbed doses have been investigated using thermal analysis, sol–gel analysis and solid state 13C nuclear magnetic Resonance (NMR). The chemical shift of POE was assigned and peak evolution as a function of radiation dose was discussed. An obviously evolution is that the peak area of 33.6 ppm decreases as a function of the increase of radiation dose, and at the same time, the peak shape broadens gradually. This indicates that the chain scission occurred between α-C and branch chain C (methine) or between C1 (the sidegroup hexyl) and branch chain C (methane) after radiation. The chain scission is severer with the increase of absorbed dose.The 13C NMR spectra of the corresponding gels confirmed the result. The variation in linewidth of the resonance at 33.6 ppm in samples of POE irradiated to different doses was attributed to information of chain, scission, new cross linking, and crystalline components.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.017
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.047
Threshold uncertainty score0.580

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0170.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.002
Science and technology studies0.0000.002
Scholarly communication0.0000.001
Open science0.0020.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.022
GPT teacher head0.365
Teacher spread0.343 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it